To enhance water resistance for catalytic ozone decomposition by fabricating H2O adsorption-site in OMS-2 tunnels
文献类型：期刊论文
| 作者 | Hong, Wei; Ma, Jinzhu; Zhu, Tianle; He, Hong ; Wang, Haining; Sun, Ye; Shen, Fangxia; Li, Xiang
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| 刊名 | APPLIED CATALYSIS B-ENVIRONMENTAL
 |
| 出版日期 | 2021-11-15 |
| 卷号 | 789页码:- |
| 关键词 | Hazardous volatile organic compounds The North China Plain Health risk assessment The heating season |
| ISSN号 | 0048-9697 |
| 英文摘要 | Severe volatile organic compound (VOC) pollution has become an urgent problem during the heating season in the North China Plain (NCP), as exposure to hazardous VOCs can lead to chronic or acute diseases. A campaign with online VOC measurements was conducted at a rural site in Wangdu, NCP during the 2018 heating season to characterize the compositions and associated sources of VOCs and to assess their potential health risks. The total concentration of VOCs with 94 identified species was 77.21 +/- 54.39 ppb. Seven source factors were identified by non-negative matrix factorization, including coal combustion (36.1%), LPG usage (21.1%), solvent usage (13.9%), biomass burning and secondary formation (142%), background (7.0%), industrial emissions (4.5%), and vehicle emissions (3.3%). The point estimate approach and Monte Carlo simulation were used to estimate the carcinogenic and non-carcinogenic risks of harzadous VOCs. The results showed that the cumulative health risk of VOCs was above the safety level. Acrolein, 1.2-dichlorprothane, 12-dichloropropane, chloroform, 1,3-butadiene, and benzene were identified as the key hazardous VOCs in Wangdu. Benzene had the highest average carcinogenic risk. Solvent usage and secondary formation were the dominant sources of adverse health effects. During the Spring Festival, most sources were sharply reduced; and VOC concentration declined by 49%. However, coal and biomass consumptions remained relatively large, probably due to heating demand. This study provides important references for the control strategies of VOCs during the heating season in heavily polluted rural areas in the NCP. (C) 2021 Elsevier B.V. All rights reserved. |
| 源URL | [https://ir.rcees.ac.cn/handle/311016/46883]  |
| 专题 | 生态环境研究中心_水污染控制实验室 |
| 作者单位 | 1.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China 2.Beihang Univ, Sch Space & Environm, Beijing Key Lab Bioinspired Energy Mat & Devices, Beijing 100191, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100085, Peoples R China |
| 推荐引用方式 GB/T 7714 | Hong, Wei,Ma, Jinzhu,Zhu, Tianle,et al. To enhance water resistance for catalytic ozone decomposition by fabricating H2O adsorption-site in OMS-2 tunnels[J]. APPLIED CATALYSIS B-ENVIRONMENTAL,2021,789:-. |
| APA | Hong, Wei.,Ma, Jinzhu.,Zhu, Tianle.,He, Hong.,Wang, Haining.,...&Li, Xiang.(2021).To enhance water resistance for catalytic ozone decomposition by fabricating H2O adsorption-site in OMS-2 tunnels.APPLIED CATALYSIS B-ENVIRONMENTAL,789,-. |
| MLA | Hong, Wei,et al."To enhance water resistance for catalytic ozone decomposition by fabricating H2O adsorption-site in OMS-2 tunnels".APPLIED CATALYSIS B-ENVIRONMENTAL 789(2021):-. |
入库方式： OAI收割
来源：生态环境研究中心
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