Heterogeneous Fenton-like reaction followed by GAC filtration improved removal efficiency of NOM and DBPs without adjusting pH
文献类型:期刊论文
作者 | Zhang, Yao; Lu, Zhili; Zhang, Zeyu; Shi, Baoyou; Hu, Chun; Lyu, Lai; Zuo, Pengxiao; Metz, Jordin; Wang, Haibo |
刊名 | SEPARATION AND PURIFICATION TECHNOLOGY |
出版日期 | 2021-04-01 |
卷号 | 260页码:- |
ISSN号 | 1383-5866 |
关键词 | Heterogeneous Fenton-like reaction Granular activated carbon filtration Natural organic matter Disinfection by-products Genotoxicity |
英文摘要 | This paper explores the removal of natural organic matter (NOM) and disinfection by-products (DBPs) in drinking water by heterogeneous Fenton-like oxidation and granular activated carbon (GAC) filtration in a pilot scale test without adjusting pH of the water. pH of the used water in this study was from 7.5 to 8.7. Comparing with conventional water treatment processes, heterogeneous Fenton-like reaction and GAC filtration increased the removal rate of dissolved organic carbon (DOC), NOM with different apparent molecular weight (AMW) (F1 F7) and with different compositions (C1-C5) to 75.11%, 88.65% and 58.73%, respectively. Moreover, heterogeneous Fenton-like reaction and GAC filtration increased the removal rate of DBPs to 88.18%. The multivariate statistical analysis indicated that haloacetic acids (HAAs) and haloketones (HKs) mainly came from fulvic-like and humic-like NOM with AMW lower than 1.5 K Da. These substances with AMW between 1.5 K Da and 3.5 K Da were the main precursors of trihalomethanes (THMs). The main precursors of halonitriles (HANs) were soluble microbial byproduct-like (SMP-like), tyrosine-like and tryptophan-like substance with the AMW between 3.5 K Da and 4.5 K Da. Overall, without adjusting pH of water, heterogeneous Fenton-like reaction and GAC filtration improved the removal efficiency of NOM and DBPs, and controlled the genotoxicity of drinking water. |
WOS研究方向 | Engineering, Chemical |
源URL | [http://ir.rcees.ac.cn/handle/311016/46219] |
专题 | 生态环境研究中心_中国科学院饮用水科学与技术重点实验室 |
作者单位 | 1.North China Univ Water Resources & Elect Power, Inst Environm & Municipal Engn, Zhengzhou 450045, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Drinking Water Sci & Technol, 18 Shuangqing Rd, Beijing 100085, Peoples R China 3.Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA 4.Guangzhou Univ, Inst Environm Res Greater Bay, Key Lab Water Qual & Conservat Pearl River Delta, Minist Educ, Guangzho 5.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 6.Rice Univ, Dept Chem, Houston, TX 77005 USA |
推荐引用方式 GB/T 7714 | Zhang, Yao,Lu, Zhili,Zhang, Zeyu,et al. Heterogeneous Fenton-like reaction followed by GAC filtration improved removal efficiency of NOM and DBPs without adjusting pH[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2021,260:-. |
APA | Zhang, Yao.,Lu, Zhili.,Zhang, Zeyu.,Shi, Baoyou.,Hu, Chun.,...&Wang, Haibo.(2021).Heterogeneous Fenton-like reaction followed by GAC filtration improved removal efficiency of NOM and DBPs without adjusting pH.SEPARATION AND PURIFICATION TECHNOLOGY,260,-. |
MLA | Zhang, Yao,et al."Heterogeneous Fenton-like reaction followed by GAC filtration improved removal efficiency of NOM and DBPs without adjusting pH".SEPARATION AND PURIFICATION TECHNOLOGY 260(2021):-. |
入库方式: OAI收割
来源:生态环境研究中心
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