Highly e ffi cient removal of selenite by electrolysis-assisted nano-zerovalent iron (nZVI): Implication for corrosion and reduction
文献类型:期刊论文
作者 | Qi, Zenglu; Liu, Ruiping; Joshi, Tista Prasai; Peng, Jianfeng; Qu, Jiuhui![]() |
刊名 | CHEMICAL ENGINEERING JOURNAL
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出版日期 | 2021-02-01 |
卷号 | 405页码:- |
关键词 | Nano zerovalent iron Selenite Corrosion products Reduction Electron transfer |
ISSN号 | 1385-8947 |
英文摘要 | In present work, an efficient purification of selenite-contaminated water using electrolysis-assisted nano zerovalent iron (E-nZVI), which achieved a removal capacity of 15.83 mg Se(IV)/g nZVI and exceeded the none assisted nZVI system by 135% was tested. Although Se(IV) removal dramatically increased with applied voltages over 2.0 V in E-nZVI system, the kinetics indicate that higher applied voltage (-4.0 V or more) and lower resistance could not result in apparent promotion on the reaction rate constant. Furthermore, the results from separate anode-cathode tests and surface-sensitive quantitative characterization reveal the synergistic effects of nZVI and cathodic reduction on elemental selenium precipitation, and nZVI corrosion aggravated by electrochemical oxidization improved removal performance in the anode chamber. In conclusion, the electrolysis assisted nZVI showed good removal efficiency of Se(IV) and is a potential water treatment method for removing reducible contaminants. |
WOS研究方向 | Engineering, Environmental ; Engineering, Chemical |
源URL | [http://ir.rcees.ac.cn/handle/311016/46220] ![]() |
专题 | 生态环境研究中心_中国科学院饮用水科学与技术重点实验室 |
作者单位 | 1.Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China 2.Chinese Acad Sci, Key Lab Drinking Water Sci & Technol, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China 3.Nepal Acad Sci & Technol, Fac Sci, Environm & Climate Study Lab, Khumaltar, Lalitpur, Nepal |
推荐引用方式 GB/T 7714 | Qi, Zenglu,Liu, Ruiping,Joshi, Tista Prasai,et al. Highly e ffi cient removal of selenite by electrolysis-assisted nano-zerovalent iron (nZVI): Implication for corrosion and reduction[J]. CHEMICAL ENGINEERING JOURNAL,2021,405:-. |
APA | Qi, Zenglu,Liu, Ruiping,Joshi, Tista Prasai,Peng, Jianfeng,&Qu, Jiuhui.(2021).Highly e ffi cient removal of selenite by electrolysis-assisted nano-zerovalent iron (nZVI): Implication for corrosion and reduction.CHEMICAL ENGINEERING JOURNAL,405,-. |
MLA | Qi, Zenglu,et al."Highly e ffi cient removal of selenite by electrolysis-assisted nano-zerovalent iron (nZVI): Implication for corrosion and reduction".CHEMICAL ENGINEERING JOURNAL 405(2021):-. |
入库方式: OAI收割
来源:生态环境研究中心
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