中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Revisiting the bioelectrochemical system based biosensor for organic sensing and the prospect on constructed wetland-microbial fuel cell

文献类型:期刊论文

作者Xu, Lei; Yu, Wenzheng; Graham, Nigel; Zhao, Yaqian
刊名CHEMOSPHERE
出版日期2021-02
卷号264页码:-
关键词Constructed wetland Bioelectrochemical system Organic sensing Normalization Anodic material Chemical shock
ISSN号0045-6535
英文摘要Bioelectrochemical system (BES) based biosensors for organic sensing has long been investigated. However, there is no uniform criterion to evaluate directly the performance of the BES based biosensors due to their different scale. Here, for the first time, we show that the normalized maximum detection range (NMDR) and normalized sensing time (NST) can potentially be used as the two criteria in BES based biosensors for organic sensing. Thereafter, the recently emerged, relatively larger scale BES (i.e. constructed wetland-microbial fuel cell, CW-MFC) was specifically examined in this study. The biocathode formation and the influence of anodic material on sensor performance were systematically evaluated. The system with metal-based anode was found to produce a more stable and quicker response (low NST) than that with carbon-based anode. Significantly, the continuous loading mode was found to greatly reduce the NMDR compared to the batch mode, and the hydraulic residence time (HRT) is the critical factor determining the NMDR. Furthermore, it was found that the electrical signals generated from the CW-MFC system were insignificantly influenced by some specific chemical disturbances, such as Cu2+ and herbicide. Therefore, normalized toxicity (NT) is suggested to be considered in BES based biosensor. However, for chemicals with higher reduction potentials (NO3- in this work), the system presented a high response, enabling its potential for monitoring NO3- in effluents or groundwater. This study can hopefully contribute to further development of the sustainable BES based biosensors in CW. (C) 2020 Elsevier Ltd. All rights reserved.
WOS研究方向Environmental Sciences
源URL[http://ir.rcees.ac.cn/handle/311016/46262]  
专题生态环境研究中心_中国科学院饮用水科学与技术重点实验室
作者单位1.Univ Coll Dublin, Ctr Water Resources Res, Sch Civil Engn, Dublin 4, Ireland
2.Imperial Coll London, Dept Civil & Environm Engn, South Kensington Campus, London SW7 2AZ, England
3.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Drinking Water Sci & Technol, Beijing 100085, Peoples R China
推荐引用方式
GB/T 7714
Xu, Lei,Yu, Wenzheng,Graham, Nigel,et al. Revisiting the bioelectrochemical system based biosensor for organic sensing and the prospect on constructed wetland-microbial fuel cell[J]. CHEMOSPHERE,2021,264:-.
APA Xu, Lei,Yu, Wenzheng,Graham, Nigel,&Zhao, Yaqian.(2021).Revisiting the bioelectrochemical system based biosensor for organic sensing and the prospect on constructed wetland-microbial fuel cell.CHEMOSPHERE,264,-.
MLA Xu, Lei,et al."Revisiting the bioelectrochemical system based biosensor for organic sensing and the prospect on constructed wetland-microbial fuel cell".CHEMOSPHERE 264(2021):-.

入库方式: OAI收割

来源:生态环境研究中心

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