Trihalomethanes formation enhanced by manganese chlorination and deposition in plastic drinking water pipes
文献类型：期刊论文
| 作者 | Yu, Ying; Li, Guiwei ; Chen, Ruya; Shi, Baoyou
|
| 刊名 | WATER RESEARCH
 |
| 出版日期 | 2021-10-01 |
| 卷号 | 204页码:- |
| 关键词 | Drinking water distribution system Trihalomethanes Manganese Organics accumulation Catalytic oxidation |
| ISSN号 | 0043-1354 |
| 英文摘要 | Residual manganese(II) in finished water undergoes further oxidation and deposition in drinking water distribution systems (DWDS), and Mn deposits can function as sites for accumulating organic and inorganic pollutants. This study aims to explore how Mn transformation and deposition affect the formation of disinfection byproducts (DBPs) in chlorinated DWDS, and trihalomethanes (THMs) was selected as a representative DBP. In a 100 mu g/L Mn system, regulated THMs (chlorinated/bromated-THMs) increased by over 20% higher than Mn-free system after 150-day operation; when 50 mu g/L iodide (I-) entered pipe systems after 150 days, iodinated THMs (I-THMs) in 100 mu g/L Mn system increased by over 30% compared with Mn-free system. These promotions were attributed primarily to the accumulation of biomolecules and organic substances by tight and hard chlorinated Mn deposits. The residence of inactivated cells and the bridging role of surface Mn(III) in Mn deposits increased the quantity of THM precursors in DWDS. Furthermore, the rapid catalytic oxidation of Mn(II) by preformed Mn oxides (MnO) x inhibited the conversion of free iodine (HOI/OI-) to iodate, resulting in the generation of more I-THMs. This study provides new insights into the DBP risks caused by Mn in DWDS. |
| WOS研究方向 | Engineering, Environmental ; Environmental Sciences ; Water Resources |
| 源URL | [http://ir.rcees.ac.cn/handle/311016/46271]  |
| 专题 | 生态环境研究中心_中国科学院饮用水科学与技术重点实验室 |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Drinking Water Sci & Technol, Beijing 100085, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yu, Ying,Li, Guiwei,Chen, Ruya,et al. Trihalomethanes formation enhanced by manganese chlorination and deposition in plastic drinking water pipes[J]. WATER RESEARCH,2021,204:-. |
| APA | Yu, Ying,Li, Guiwei,Chen, Ruya,&Shi, Baoyou.(2021).Trihalomethanes formation enhanced by manganese chlorination and deposition in plastic drinking water pipes.WATER RESEARCH,204,-. |
| MLA | Yu, Ying,et al."Trihalomethanes formation enhanced by manganese chlorination and deposition in plastic drinking water pipes".WATER RESEARCH 204(2021):-. |
入库方式： OAI收割
来源：生态环境研究中心
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