Fabrication of gamma-Al2O3 Nanoarrays on Aluminum Foam Assisted by Hydroxide for Monolith Catalysts
文献类型：期刊论文
| 作者 | Peng, Shengpan2; Ma, Ziran2; Ma, Jing2; Han, Zhihua2; Wang, Hongyan2; Wang, Baodong2; Zhao, Feng1; Li, Ge2 |
| 刊名 | ACS OMEGA
 |
| 出版日期 | 2022-12-28 |
| 页码 | 9 |
| ISSN号 | 2470-1343 |
| DOI | 10.1021/acsomega.2c07237 |
| 英文摘要 | Heat distribution and good adhesion of the washcoat on monolith catalysts are critical to improving catalytic activity and long-term stability. Compared with cordierite, metal foam presents a high thermal conductivity coefficient. Also, the availability of "washcoat" in situ grown on metal substrates opens the door to eliminating the problem of coating peeling. Generally, hydrothermal or thermal methods are used for the fabrication of in situ grown washcoat on metal substrates. In this research, the aluminum foam monolith vertically aligned Al2O3 nanowire array is successfully prepared at ambient temperature in an alkaline solution for the first time. Furthermore, the Pt-loaded Al2O3 nanowire array (0.5 gPt/Lmonolith) is applied to C2H4 degradation. The catalyst converts 90% C2H4 at 147 degrees C with a gas hourly space velocity (GHSV) of 20,000 h-1. And a little decrease (1%) is observed in catalytic activity, even in 15 vol % water vapors. The catalysts show good thermal stability and water resistance property over 36 h at 300 degrees C. Above all, this study presents a simple way of in situ growth of washcoat on metal-substrate monolith with potentially scaled manufacturing. And the monolith catalyst shows good catalytic performance on C2H4, which can be applied for volatile organic compound treatment. |
| WOS关键词 | AL ; PLATINUM ; BOEHMITE ; TEMPERATURE ; MORPHOLOGY ; CONVERSION ; STABILITY ; MECHANISM ; OXIDATION ; SURFACES |
| 资助项目 | Science and Technology Project of China Energy Investment[ST930021005C] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000912773500001 |
| 资助机构 | Science and Technology Project of China Energy Investment |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/56767]  |
| 通讯作者 | Wang, Baodong |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China 2.Natl Inst Clean & Low Carbon Energy, Beijing 102211, Peoples R China |
| 推荐引用方式 GB/T 7714 | Peng, Shengpan,Ma, Ziran,Ma, Jing,et al. Fabrication of gamma-Al2O3 Nanoarrays on Aluminum Foam Assisted by Hydroxide for Monolith Catalysts[J]. ACS OMEGA,2022:9. |
| APA | Peng, Shengpan.,Ma, Ziran.,Ma, Jing.,Han, Zhihua.,Wang, Hongyan.,...&Li, Ge.(2022).Fabrication of gamma-Al2O3 Nanoarrays on Aluminum Foam Assisted by Hydroxide for Monolith Catalysts.ACS OMEGA,9. |
| MLA | Peng, Shengpan,et al."Fabrication of gamma-Al2O3 Nanoarrays on Aluminum Foam Assisted by Hydroxide for Monolith Catalysts".ACS OMEGA (2022):9. |
入库方式： OAI收割
来源：过程工程研究所
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