Catalytic template assisted interfacial polymerization for high-performance acid-resistant membrane preparation
文献类型：期刊论文
| 作者 | Cao, Yang2,3; Wan, Yinhua2,3,4; Chen, Chulong5; Luo, Jianquan1,2,3 |
| 刊名 | AICHE JOURNAL
 |
| 出版日期 | 2023-01-24 |
| 页码 | 11 |
| 关键词 | acid-resistant membrane catalytic template interfacial polymerization poly(amide-sulfonamide) thin-film composite membrane |
| ISSN号 | 0001-1541 |
| DOI | 10.1002/aic.18038 |
| 英文摘要 | Highly permeable acid-resistant nanofiltration (NF) membranes are of critical significance for the efficient treatment of acidic streams. Enhancing permeability while maintaining the high solute rejection of acid-resistant NF membranes remains a great challenge due to the low reactivity of monomers. In this work, a novel catalytic template assisted interfacial polymerization (IP) strategy of 3-aminobenzenesulfonamide (ABSA) and trimesoyl chloride (TMC) was provided to prepare a poly(amide-sulfonamide) membrane. Aminopyridine doped graphene quantum dots rich in acylation catalytic sites and ZIF-8 nanoparticles are co-loaded on a substrate as template. Benefiting from the enhanced phase integrity and self-inhibition effect of the template assisted IP process, the resulting ultra-thin acid-resistant membrane exhibits an excellent water permeance (20.4 Lm(-2)h(-1)bar(-1)) with a high Na2SO4 rejection of 90.5%, which outperforms almost all the reported acid-resistant NF membranes. Our work paves a versatile way for synthesis of special separation membranes. |
| WOS关键词 | FILM COMPOSITE MEMBRANE ; NANOFILTRATION MEMBRANES ; NAPHTHALENE-1,3,6-TRISULFONYLCHLORIDE NTSC ; LAYER ; PH ; NANOFILMS ; STABILITY ; CHLORIDE |
| 资助项目 | National Key Research and Development Program of China[2021YFC3201402] ; Province Key Research and Development Program of Shandong[2019JZZY010348] ; ZheJiang MEY Membrane Technology Co., Ltd |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000922244900001 |
| 出版者 | WILEY |
| 资助机构 | National Key Research and Development Program of China ; Province Key Research and Development Program of Shandong ; ZheJiang MEY Membrane Technology Co., Ltd |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/56918]  |
| 通讯作者 | Luo, Jianquan |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing, Peoples R China 3.Univ Chinese Acad Sci, Sch Chem Engn, Beijing, Peoples R China 4.Chinese Acad Sci, Ganjiang Innovat Acad, Ganzhou, Peoples R China 5.ZheJiang MEY Membrane Technol CO LTD, Hangzhou, Peoples R China |
| 推荐引用方式 GB/T 7714 | Cao, Yang,Wan, Yinhua,Chen, Chulong,et al. Catalytic template assisted interfacial polymerization for high-performance acid-resistant membrane preparation[J]. AICHE JOURNAL,2023:11. |
| APA | Cao, Yang,Wan, Yinhua,Chen, Chulong,&Luo, Jianquan.(2023).Catalytic template assisted interfacial polymerization for high-performance acid-resistant membrane preparation.AICHE JOURNAL,11. |
| MLA | Cao, Yang,et al."Catalytic template assisted interfacial polymerization for high-performance acid-resistant membrane preparation".AICHE JOURNAL (2023):11. |
入库方式： OAI收割
来源：过程工程研究所
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