Bioelectrocatalysis for CO2 reduction: recent advances and challenges to develop a sustainable system for CO2 utilization
文献类型：期刊论文
| 作者 | Luan, Likun1,2; Ji, Xiuling1; Guo, Boxia1,2; Cai, Jinde1; Dong, Wanrong1; Huang, Yuhong1; Zhang, Suojiang1 |
| 刊名 | BIOTECHNOLOGY ADVANCES
 |
| 出版日期 | 2023-03-01 |
| 卷号 | 63页码:28 |
| 关键词 | CO 2 reduction Bioelectrocatalysis Electron transfer Photo-electrocatalysis |
| ISSN号 | 0734-9750 |
| DOI | 10.1016/j.biotechadv.2023.108098 |
| 英文摘要 | Activation and turning CO2 into value added products is a promising orientation to address environmental issues caused by CO2 emission. Currently, electrocatalysis has a potent well-established role for CO2 reduction with fast electron transfer rate; but it is challenged by the poor selectivity and low faradic efficiency. On the other side, biocatalysis, including enzymes and microbes, has been also employed for CO2 conversion to target Cn products with remarkably high selectivity; however, low solubility of CO2 in the liquid reaction phase seriously affects the catalytic efficiency. Therefore, a new synergistic role in bioelectrocatalysis for CO2 reduction is emerging thanks to its outstanding selectivity, high faradic efficiency, and desirable valuable Cn products under mild condition that are surveyed in this review. Herein, we comprehensively discuss the results already obtained for the inte-gration craft of enzymatic-electrocatalysis and microbial-electrocatalysis technologies. In addition, the intrinsic nature of the combination is highly dependent on the electron transfer. Thus, both direct electron transfer and mediated electron transfer routes are modeled and concluded. We also explore the biocompatibility and syn-ergistic effects of electrode materials, which emerge in combination with tuned enzymes and microbes to improve catalytic performance. The system by integrating solar energy driven photo-electrochemical technics with bio-catalysis is further discussed. We finally highlight the significant findings and perspectives that have provided strong foundations for the remarkable development of green and sustainable bioelectrocatalysis for CO2 reduction, and that offer a blueprint for Cn valuable products originate from CO2 under efficient and mild conditions. |
| WOS关键词 | DIRECT ELECTRON-TRANSFER ; CARBON-MONOXIDE DEHYDROGENASE ; CONTAINING FORMATE DEHYDROGENASE ; SYNTHETIC ENZYMATIC PATHWAY ; NAD(+)/NADH REDOX COUPLES ; METAL-ORGANIC FRAMEWORKS ; MICROBIAL FUEL-CELLS ; ELECTROCHEMICAL CONVERSION ; DIRECTED EVOLUTION ; NADH REGENERATION |
| 资助项目 | National Key Research and Development Program[2021YFC2104200] ; "Transformational Technologies for Clean Energy and Demonstration" Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21000000] ; National Natural Science Foundation of China[22078346] ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China[21921005] ; Beijing Nova Program of Science and Technology[Z201100006820141] ; Beijing Nova Program of Science and Technology[Z211100002121164] ; CAS Project for Young Scientists in Basic Research[YSBR- 072] |
| WOS研究方向 | Biotechnology & Applied Microbiology |
| 语种 | 英语 |
| WOS记录号 | WOS:000924660600001 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Key Research and Development Program ; "Transformational Technologies for Clean Energy and Demonstration" Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China ; Beijing Nova Program of Science and Technology ; CAS Project for Young Scientists in Basic Research |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/56948]  |
| 通讯作者 | Huang, Yuhong; Zhang, Suojiang |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn,State Key Lab Multip, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sino Danish Coll, Beijing 101408, Peoples R China |
| 推荐引用方式 GB/T 7714 | Luan, Likun,Ji, Xiuling,Guo, Boxia,et al. Bioelectrocatalysis for CO2 reduction: recent advances and challenges to develop a sustainable system for CO2 utilization[J]. BIOTECHNOLOGY ADVANCES,2023,63:28. |
| APA | Luan, Likun.,Ji, Xiuling.,Guo, Boxia.,Cai, Jinde.,Dong, Wanrong.,...&Zhang, Suojiang.(2023).Bioelectrocatalysis for CO2 reduction: recent advances and challenges to develop a sustainable system for CO2 utilization.BIOTECHNOLOGY ADVANCES,63,28. |
| MLA | Luan, Likun,et al."Bioelectrocatalysis for CO2 reduction: recent advances and challenges to develop a sustainable system for CO2 utilization".BIOTECHNOLOGY ADVANCES 63(2023):28. |
入库方式： OAI收割
来源：过程工程研究所
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