Regeneration kinetics of spent FCC catalyst via coke gasification in a micro fluidized bed
文献类型:会议论文
作者 | Zhang, Yuming1,2; Sun, Guogang1; Gao, Shiqiu2; Xu, Guangwen2 |
出版日期 | 1905-07-07 |
会议日期 | May 19, 2014 - May 22, 2014 |
会议地点 | Beijing, China |
关键词 | Kinetic parameters - Fluidized bed process - Fluid catalytic cracking - Coke - Activation energy - Gasification - Chemical reactors |
卷号 | 102 |
DOI | 10.1016/j.proeng.2015.01.312 |
页码 | 1758-1765 |
英文摘要 | In the present study, the spent fluid catalytic cracking (FCC) catalyst is regenerated via coke gasification instead of combustion in a micro fluidized bed reactor to investigate its reaction characteristics and kinetic parameters. The reaction rate first increased with carbon conversion ratio and then slowly decreased when reaching the peak. H2 and CO was found to be over 70 vol.% in the gasification gas. Two reaction models, homogenous model (HM) and shrinking core model (SCM) were used to calculate the kinetic parameters of catalyst regeneration, finding that HM had better fitting relevance for the data than SCM. The activation energy from these two models was close to each other, that is, about 150 kJ.mol-1 for the coke gasification over FCC catalyst. 漏 2015 Published by Elsevier Ltd. |
项目编号 | The study was conducted with the research programs supported by Science Foundation of China University of Petroleum, Beijing (No. 2462013YJRC021), National Instrumentation Grant Program (2011YQ120039), National Basic Research Program of China (973 Program, NO. 2012CB224801). Acknowledgements are also extended to Mr. Deping Yu for his help on the experiments. |
资助机构 | Elsevier Ltd |
会议录 | 7th World Congress on Particle Technology, WCPT 2014
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学科主题 | Fluidized Beds |
源URL | [http://ir.ipe.ac.cn/handle/122111/59341] ![]() |
作者单位 | 1.State Key Laboratory of Heavy Oil Processing, China University of Petroleum-Beijing, Beijing; 102249, China 2.State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing; 100190, China |
推荐引用方式 GB/T 7714 | Zhang, Yuming,Sun, Guogang,Gao, Shiqiu,et al. Regeneration kinetics of spent FCC catalyst via coke gasification in a micro fluidized bed[C]. 见:. Beijing, China. May 19, 2014 - May 22, 2014. |
入库方式: OAI收割
来源:过程工程研究所
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