Artificial photosynthesis systems for solar energy conversion and storage: platforms and their realities
文献类型：期刊论文
| 作者 | Wang, Zhenfu1; Hu, Yang1; Zhang, Songping2; Sun, Yan1 |
| 刊名 | Chemical Society Reviews
 |
| 出版日期 | 2022-07-11 |
| 卷号 | 51期号:15页码:6704-6737 |
| ISSN号 | 3060012 |
| 关键词 | Artificial photosynthesis - Energy utilization - Solar energy conversion |
| DOI | 10.1039/d1cs01008e |
| 英文摘要 | In natural photosynthesis, photosynthetic organisms such as green plants realize efficient solar energy conversion and storage by integrating photosynthetic components on the thylakoid membrane of chloroplasts. Inspired by natural photosynthesis, researchers have developed many artificial photosynthesis systems (APS's) that integrate various photocatalysts and biocatalysts to convert and store solar energy in the fields of resource, environment, food, and energy. To improve the system efficiency and reduce the operation cost, reaction platforms are introduced in APS's since they allow for great stability and continuous processing. A systematic understanding of how a reaction platform affects the performance of artificial photosynthesis is conducive for designing an APS with superb solar energy utilization. In this review, we discuss the recent APS's researches, especially those confined on/in platforms. The importance of different platforms and their influences on APS's performance are emphasized. Generally, confined platforms can enhance the stability and repeatability of both photocatalysts and biocatalysts in APS's as well as improve the photosynthetic performance due to the proximity effect. For functional platforms that can participate in the artificial photosynthesis reactions as active parts, a high integration of APS's components on/in these platforms can lead to efficient electron transfer, enhanced light-harvesting, or synergistic catalysis, resulting in superior photosynthesis performance. Therefore, the integration of APS's components is beneficial for the transfer of substrates and photoexcited electrons in artificial photosynthesis. We finally summarize the current challenges of APS's development and further efforts on the improvement of APS's. 漏 2022 The Royal Society of Chemistry. |
| 学科主题 | Solar Energy |
| 项目编号 | This work was funded by the National Key Research and Development Program of China (grant no. 2021YFC2102801) and the National Natural Science Foundation of China (no. 21621004). |
| 出版者 | Royal Society of Chemistry |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/61231]  |
| 作者单位 | 1.Department of Biochemical Engineering, School of Chemical Engineering and Technology and Key Laboratory of Systems Bioengineering and Frontiers Science Center for Synthetic Biology (Ministry of Education), Tianjin University, Tianjin; 300350, China 2.State Key Laboratory of Biochemical Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing; 100190, China |
| 推荐引用方式 GB/T 7714 | Wang, Zhenfu,Hu, Yang,Zhang, Songping,et al. Artificial photosynthesis systems for solar energy conversion and storage: platforms and their realities[J]. Chemical Society Reviews,2022,51(15):6704-6737. |
| APA | Wang, Zhenfu,Hu, Yang,Zhang, Songping,&Sun, Yan.(2022).Artificial photosynthesis systems for solar energy conversion and storage: platforms and their realities.Chemical Society Reviews,51(15),6704-6737. |
| MLA | Wang, Zhenfu,et al."Artificial photosynthesis systems for solar energy conversion and storage: platforms and their realities".Chemical Society Reviews 51.15(2022):6704-6737. |
入库方式： OAI收割
来源：过程工程研究所
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