Experimental study on gas holdup and bubble behavior in carbon capture systems with ionic liquid
文献类型：期刊论文
| 作者 | Zhang, Xin1,2; Dong, Haifeng1; Huang, Ying1,2; Li, Chunshan1; Zhang, Xiangping1,3 |
| 刊名 | CHEMICAL ENGINEERING JOURNAL
 |
| 出版日期 | 2012-10-15 |
| 卷号 | 209期号:0页码:607-615 |
| 关键词 | Ionic liquids Carbon capture Gas holdup Bubble size distribution Sauter diameter Interfacial area |
| ISSN号 | 1385-8947 |
| 通讯作者 | Zhang, XP |
| 英文摘要 | Ionic liquids (ILs) have been widely considered as potential green solvents for CO2 capture, and many promising ionic liquids have been synthesized and reported. However, knowledge related to the hydrodynamics of CO2 absorption with ionic liquids especially the bubble behavior is still scarce compared with the conventional molecular solvents. In this study, it is the first time to discuss the multi-bubble behavior in a carbon capture system with ionic liquid by using a high speed image pick-up system. The bubble behavior, such as bubble size distribution, total gas holdup, Sauter diameter and interfacial area at different operating conditions are investigated. The experimental results show that the bubble diameter of CO2-[bmim][BE4] system is smaller than that of N-2-[bmim][BF4] system. The bubble diameter increases as the gas superficial velocity increases and the height along the axis of the column rises, but decreases with the increase of the temperature. The total gas holdup in [bmim][BF4] increases with the increase of the system temperature due to the decrease of the ionic liquid viscosity. In addition, the gas superficial velocity improves the total gas holdup due to the higher gas momentum favors the formation of small bubbles. A new correlation based on the experimental data is proposed for the prediction of Sauter diameter in gas-ionic liquid systems. The prediction results calculated by the new correlation are in good agreement with the experimental data with a relative error less than 6%. (C) 2012 Elsevier B.V. All rights reserved. |
| WOS标题词 | Science & Technology ; Technology |
| 类目[WOS] | Engineering, Environmental ; Engineering, Chemical |
| 研究领域[WOS] | Engineering |
| 关键词[WOS] | MASS-TRANSFER ; SIZE DISTRIBUTION ; COLUMN REACTORS ; SURFACE-TENSION ; FLOW REGIME ; BREAK-UP ; DIAMETER ; CO2 ; HYDRODYNAMICS ; DISTRIBUTIONS |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000311190500071 |
| 公开日期 | 2013-10-11 |
| 版本 | 出版稿 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/3155]  |
| 专题 | 过程工程研究所_多相复杂系统国家重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Grad Univ, Coll Chem & Chem Engn, Beijing 100049, Peoples R China 3.Norwegian Univ Sci & Technol, Dept Energy & Proc Engn, NO-7491 Trondheim, Norway |
| 推荐引用方式 GB/T 7714 | Zhang, Xin,Dong, Haifeng,Huang, Ying,et al. Experimental study on gas holdup and bubble behavior in carbon capture systems with ionic liquid[J]. CHEMICAL ENGINEERING JOURNAL,2012,209(0):607-615. |
| APA | Zhang, Xin,Dong, Haifeng,Huang, Ying,Li, Chunshan,&Zhang, Xiangping.(2012).Experimental study on gas holdup and bubble behavior in carbon capture systems with ionic liquid.CHEMICAL ENGINEERING JOURNAL,209(0),607-615. |
| MLA | Zhang, Xin,et al."Experimental study on gas holdup and bubble behavior in carbon capture systems with ionic liquid".CHEMICAL ENGINEERING JOURNAL 209.0(2012):607-615. |
入库方式： OAI收割
来源：过程工程研究所
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