Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides
文献类型：期刊论文
| 作者 | Jiang, Ru-Jian1,2; Cao, Yi1,2; Geng, Wan-Rong3; Zhu, Mei-Xiong1,2; Tang, Yun-Long1; Zhu, Yin-Lian3; Wang, Yujia1; Gong, Fenghui1,2; Liu, Su-Zhen1,2; Chen, Yu-Ting1,2 |
| 刊名 | NANO LETTERS
 |
| 出版日期 | 2023-02-01 |
| 页码 | 8 |
| ISSN号 | 1530-6984 |
| 关键词 | antiferroelectric lead zirconate consecutive phase transformation short-period phase scanning transmission electron microscopy |
| DOI | 10.1021/acs.nanolett.2c04972 |
| 通讯作者 | Tang, Yun-Long(yltang@imr.ac.cn) ; Zhu, Yin-Lian(zhuyinlian@sslab.org.cn) |
| 英文摘要 | Antiferroelectrics characterized by voltage-driven reversible transitions between antiparallel and parallel polarity are promising for cutting-edge electronic and electrical power applications. Wide-ranging explorations revealing the macroscopic performances and microstructural characteristics of typical antiferroelectric systems have been conducted. However, the underlying mechanism has not yet been fully unraveled, which depends largely on the atomistic processes. Herein, based on atomic-resolution transmission electron microscopy, the deterministic phase transition pathway along with the underlying lattice-by-lattice details in lead zirconate thin films was elucidated. Specifically, we identified a new type of ferrielectric-like dipole configuration with both angular and amplitude modulations, which plays the role of a precursor for a subsequent antiferroelectric to ferroelectric transformation. With the participation of the ferrielectric-like phase, the phase transition pathways driven by the phase boundary have been revealed. We provide new insights into the consecutive phase transformation in low-dimensional lead zirconate, which thus would promote potential antiferroelectric-based multifunctional devices. |
| 资助项目 | National Natural Science Foundation of China[51971223] ; National Natural Science Foundation of China[51922100] ; National Natural Science Foundation of China[52122101] ; Key Research Program of Frontier Sciences CAS[QYZDJ-SSW-JSC010] ; Shenyang National Laboratory for Materials Science[L2019R06] ; Shenyang National Laboratory for Materials Science[L2019R08] ; Shenyang National Laboratory for Materials Science[L2019F01] ; Shenyang National Laboratory for Materials Science[L2019F13] ; Scientific Instrument Developing Project of CAS[YJKYYQ20200066] ; Youth Innovation Promotion Association CAS[Y202048] ; Youth Innovation Promotion Association CAS[2021187] ; Guangdong Basic and Applied Basic Research Foundation[2021A1515110291] ; China Postdoctoral Science Foundation[2022T150690] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000927041400001 |
| 资助机构 | National Natural Science Foundation of China ; Key Research Program of Frontier Sciences CAS ; Shenyang National Laboratory for Materials Science ; Scientific Instrument Developing Project of CAS ; Youth Innovation Promotion Association CAS ; Guangdong Basic and Applied Basic Research Foundation ; China Postdoctoral Science Foundation |
| 源URL | [http://ir.imr.ac.cn/handle/321006/175130]  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Tang, Yun-Long; Zhu, Yin-Lian |
| 作者单位 | 1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 2.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 3.Bay Area Ctr Electron Microscopy, Songshan Lake Mat Lab, Dongguan 523808, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jiang, Ru-Jian,Cao, Yi,Geng, Wan-Rong,et al. Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides[J]. NANO LETTERS,2023:8. |
| APA | Jiang, Ru-Jian.,Cao, Yi.,Geng, Wan-Rong.,Zhu, Mei-Xiong.,Tang, Yun-Long.,...&Ma, Xiu-Liang.(2023).Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides.NANO LETTERS,8. |
| MLA | Jiang, Ru-Jian,et al."Atomic Insight into the Successive Antiferroelectric-Ferroelectric Phase Transition in Antiferroelectric Oxides".NANO LETTERS (2023):8. |
入库方式： OAI收割
来源：金属研究所
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