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Study on anisotropic oxide formation rate in the initial corrosion stage of 90Cu-10Ni alloy in alkaline NaCl solution by experiments and first-principles calculation

文献类型：期刊论文

作者Yi, Xuening3,4; Zhang, Lianji5; Ma, Aili2,3; Zhang, Lianmin3; Cao, Shuo1; Hu, Qingmiao1; Hu, Lingyue6; Zheng, Yugui2,3
刊名CORROSION SCIENCE
出版日期2022-12-01
卷号209页码:14
关键词Alloy AFM Raman spectroscopy Crystallographic anisotropy First-principles calculation
ISSN号0010-938X
DOI10.1016/j.corsci.2022.110768
通讯作者Ma, Aili(alma@imr.ac.cn) ; Zheng, Yugui(ygzheng@imr.ac.cn)
英文摘要Corrosion of 90Cu-10Ni alloy is related to oxide film formed in seawater. We characterize the initial oxides formed on different grains immersed in alkaline NaCl solution and reveal grain-orientation dependent Cu2O formation rate of (001) < (101) < (111) which causes Volta potential reversal among grains. We also implement the first-principles calculation on (001), (101) and (111) surfaces with monoatomic steps and demonstrate that anisotropic Cl adsorbing capacity and Cu dissolving capacity are responsible for different oxidation rates. Our results provide insights to optimize corrosion properties of conventional alloys on the concept of homogenizing oxide film by tailoring surface texture.
资助项目National Natural Science Foundations of China[51871226] ; National Natural Science Foundations of China[52175192] ; CAS Key laboratory of Nuclear Materials and Safety Assessment[2021NMSAKF03] ; National Supercomputing Center in Zhengzhou
WOS研究方向Materials Science ; Metallurgy & Metallurgical Engineering
语种英语
WOS记录号WOS:000883743500002
出版者PERGAMON-ELSEVIER SCIENCE LTD
资助机构National Natural Science Foundations of China ; CAS Key laboratory of Nuclear Materials and Safety Assessment ; National Supercomputing Center in Zhengzhou
源URL[http://ir.imr.ac.cn/handle/321006/176674]  
专题金属研究所_中国科学院金属研究所
通讯作者Ma, Aili; Zheng, Yugui
作者单位1.Chinese Acad Sci, Inst Met Res, 72 Wenhua Rd, Shenyang 110016, Peoples R China
2.Chinese Acad Sci, Inst Met Res, 62 Wencui Rd, Shenyang 110016, Peoples R China
3.Chinese Acad Sci, Inst Met Res, CAS Key Lab Nucl Mat & Safety Assessment, 62 Wencui Rd, Shenyang 110016, Peoples R China
4.Yantai Univ, Sch Nucl Equipment & Nucl Engn, Yantai 264005, Peoples R China
5.Zhengzhou Univ, Sch Mat Sci & Engn, 100 Sci Ave, Zhengzhou 450001, Peoples R China
6.Wuhan Second Ship Design & Res Inst, 450 Zhongshan Rd, Wuhan 430064, Peoples R China
推荐引用方式
GB/T 7714		 Yi, Xuening,Zhang, Lianji,Ma, Aili,et al. Study on anisotropic oxide formation rate in the initial corrosion stage of 90Cu-10Ni alloy in alkaline NaCl solution by experiments and first-principles calculation[J]. CORROSION SCIENCE,2022,209:14.
APA Yi, Xuening.,Zhang, Lianji.,Ma, Aili.,Zhang, Lianmin.,Cao, Shuo.,...&Zheng, Yugui.(2022).Study on anisotropic oxide formation rate in the initial corrosion stage of 90Cu-10Ni alloy in alkaline NaCl solution by experiments and first-principles calculation.CORROSION SCIENCE,209,14.
MLA Yi, Xuening,et al."Study on anisotropic oxide formation rate in the initial corrosion stage of 90Cu-10Ni alloy in alkaline NaCl solution by experiments and first-principles calculation".CORROSION SCIENCE 209(2022):14.

入库方式： OAI收割

来源：金属研究所

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