CO2-Brine-rock interaction and sequestration capacity in carbonate reservoirs of the Tahe Oilfield, Xinjiang, China
文献类型:期刊论文
作者 | Tan, Yongsheng; Li, Qi; Xu, Liang; Xu, Lifeng; Yu, Tao; Cao, Xiaomin |
刊名 | GREENHOUSE GASES-SCIENCE AND TECHNOLOGY |
出版日期 | 2022-10-10 |
卷号 | 12期号:5页码:642 |
ISSN号 | 2152-3878 |
关键词 | CO2-brine-rock interaction CO2 solubility wettability alteration carbonate reservoir CO2 sequestration capacity Tahe oilfield |
英文摘要 | The characteristics of each carbonate reservoir are greatly different, and current databases are insufficient to support engineering scheme design and optimization of carbon dioxide (CO2) sequestration and enhanced oil recovery. In this paper, the behavior of CO2-brine-rock interactions was investigated under supercritical CO2 (50 degrees C and 8.5 MPa) conditions. Five experiments were carried out, including CO2 solubility in brine, mass loss analysis by static reaction of CO2-brine-rock, mineralogical composition analysis by X-ray diffraction (XRD), core surface morphology analysis by scanning electron microscopy (SEM), and wettability alteration by contact angle analysis. The experimental results showed that: (a) the CO2 solubility in brine increases with increasing pressure, but it increases slowly and gradually reaches equilibrium; (b) the mass loss of carbonate increases with reaction time, but its increments decrease with reaction time; (c) the calcite content gradually decreases and the quartz content slightly increases with reaction time, as evidenced by XRD analysis; (d) based on SEM image analysis, calcite was dissolved into brine by carbonic acid to make the pores larger, and then subsequent precipitation made the pores smaller; and (e) the carbonate rock surface became more water-wet after CO2-brine-rock interaction experiments due to surface corrosion and increased quartz content. Using the experimental results, a mathematical model was developed to predict CO2 sequestration capacity under reservoir conditions. The results suggest that CO2 solubility in brine was the main aspect compared with mineral trapping in carbonate reservoirs, and CO2 sequestration capacity increased with increasing temperature and pressure. (c) 2022 Society of Chemical Industry and John Wiley & Sons, Ltd. |
学科主题 | Energy & Fuels ; Engineering ; Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | WILEY PERIODICALS, INC |
WOS记录号 | WOS:000850913700001 |
源URL | [http://119.78.100.198/handle/2S6PX9GI/34737] |
专题 | 中科院武汉岩土力学所 |
作者单位 | 1.Chinese Academy of Sciences; Wuhan Institute of Rock & Soil Mechanics, CAS; 2.Chinese Academy of Sciences; University of Chinese Academy of Sciences, CAS |
推荐引用方式 GB/T 7714 | Tan, Yongsheng,Li, Qi,Xu, Liang,et al. CO2-Brine-rock interaction and sequestration capacity in carbonate reservoirs of the Tahe Oilfield, Xinjiang, China[J]. GREENHOUSE GASES-SCIENCE AND TECHNOLOGY,2022,12(5):642. |
APA | Tan, Yongsheng,Li, Qi,Xu, Liang,Xu, Lifeng,Yu, Tao,&Cao, Xiaomin.(2022).CO2-Brine-rock interaction and sequestration capacity in carbonate reservoirs of the Tahe Oilfield, Xinjiang, China.GREENHOUSE GASES-SCIENCE AND TECHNOLOGY,12(5),642. |
MLA | Tan, Yongsheng,et al."CO2-Brine-rock interaction and sequestration capacity in carbonate reservoirs of the Tahe Oilfield, Xinjiang, China".GREENHOUSE GASES-SCIENCE AND TECHNOLOGY 12.5(2022):642. |
入库方式: OAI收割
来源:武汉岩土力学研究所
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