Simultaneous removal of toluene and chlorobenzene in a nonthermal plasma-catalysis reactor packed with Fe1-Mn1/gamma-Al2O3
文献类型：期刊论文
| 作者 | Qin, Linbo; Zhao, Bo; Chen, Wangsheng; Han, Yuxin; Wan, Yong; Liu, Lei; Lu, Haijun; Han, Jun |
| 刊名 | JOURNAL OF CLEANER PRODUCTION
 |
| 出版日期 | 2022-08-20 |
| 卷号 | 363 |
| ISSN号 | 0959-6526 |
| 关键词 | Non-thermal plasma Fe-Mn ?-Al 2 O 3 Simultaneous removal Kinetic Removal pathway |
| 英文摘要 | Toluene and chlorobenzene are the representative aromatic VOCs and chlorinated VOCs coexisted in the exhaust gases. In this study, the removal of the single pollutant (toluene or chlorobenzene) and the multipollutants (toluene and chlorobenzene) were studied in a nonthermal plasma reactor packed with Fe1-Mn1/gamma-Al2O3. Meanwhile, the toxic by-products, reaction kinetic and degradation pathway were also discussed. The results indicated that the multipollutants removal had a negative impact on toluene and chlorobenzene conversion. Meanwhile, O3 and NOx generated from simultaneous removal were also higher than that obtained from single pollutant (toluene or chlorobenzene) removal in the nonthermal plasma reactor packed with the Fe1-Mn1/ gamma-Al2O3. The reaction rates for toluene or chlorobenzene removal were 0.00168 s-1 and 0.00134 s-1, respectively. While the reaction rates of toluene and chlorobenzene during the simultaneous removal were respectively reduced to 0.00111 s-1 and 0.00099 s-1 due to the interaction between toluene and chlorobenzene. Finally, the possible removal pathway of simultaneous removal of toluene and chlorobenzene in the plasma reactor coupled with Fe1-Mn1/gamma-Al2O3 was also proposed based on the organic intermediates identified by GC/MS. |
| 学科主题 | Science & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| 出版者 | ELSEVIER SCI LTD |
| WOS记录号 | WOS:000821923000006 |
| 源URL | [http://119.78.100.198/handle/2S6PX9GI/35028]  |
| 专题 | 中科院武汉岩土力学所 |
| 作者单位 | 1.Wuhan University of Science & Technology; Wuhan University of Science & Technology; 2.Chinese Academy of Sciences; Wuhan Institute of Rock & Soil Mechanics, CAS |
| 推荐引用方式 GB/T 7714 | Qin, Linbo,Zhao, Bo,Chen, Wangsheng,et al. Simultaneous removal of toluene and chlorobenzene in a nonthermal plasma-catalysis reactor packed with Fe1-Mn1/gamma-Al2O3[J]. JOURNAL OF CLEANER PRODUCTION,2022,363. |
| APA | Qin, Linbo.,Zhao, Bo.,Chen, Wangsheng.,Han, Yuxin.,Wan, Yong.,...&Han, Jun.(2022).Simultaneous removal of toluene and chlorobenzene in a nonthermal plasma-catalysis reactor packed with Fe1-Mn1/gamma-Al2O3.JOURNAL OF CLEANER PRODUCTION,363. |
| MLA | Qin, Linbo,et al."Simultaneous removal of toluene and chlorobenzene in a nonthermal plasma-catalysis reactor packed with Fe1-Mn1/gamma-Al2O3".JOURNAL OF CLEANER PRODUCTION 363(2022). |
入库方式： OAI收割
来源：武汉岩土力学研究所
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