中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Effect of H2S content on relative permeability and capillary pressure characteristics of acid gas/brine/rock systems: A review

文献类型:期刊论文

作者Zhang, Xiaoyan1,2; Li, Qi1,2; Simon, Mathias3; Zheng, Guodong4; Tan, Yongsheng1,2
刊名JOURNAL OF ROCK MECHANICS AND GEOTECHNICAL ENGINEERING
出版日期2022-12-01
卷号14期号:6页码:2003
关键词Acid gas geological sequestration Relative permeability Capillary pressure H2S content Wettability Interfacial tension
ISSN号1674-7755
英文摘要Geological storage of acid gas has been identified as a promising approach to reduce atmospheric carbon dioxide (CO2), hydrogen sulfide (H2S) and alleviate public concern resulting from the sour gas production. A good understanding of the relative permeability and capillary pressure characteristics is crucial to predict the process of acid gas injection and migration. The prediction of injection and redistribution of acid gas is important to determine storage capacity, formation pressure, plume extent, shape, and leakage potential. Herein, the existing experimental data and theoretical models were reviewed to gain a better understanding of the issue how the H2S content affects gas density, gas viscosity, interfacial tension, wettability, relative permeability and capillary pressure characteristics of acid gas/brine/rock systems. The densities and viscosities of the acid gas with different H2S mole fractions are both temperature- and pressure-dependent, which vary among the gas, liquid and supercritical phases. Water/acid gas interfacial tension decreases strongly with increasing H2S content. For mica and clean quartz, water contact angle increases with increasing H2S mole fraction. In particular, wettability reversal of mica to a H2S -wet behavior occurs in the presence of dense H2S. The capillary pressure increases with decreasing contact angle. At a given saturation, the relative permeability of a fluid is higher when the fluid is nonwetting. The capillary pressure decreases with decreasing interfacial tension at a given saturation. However, the existing datasets do not show a consistent link between capillary number and relative permeability. The capillary pressure decreases with increasing H2S mole fraction. However, there is no consensus on the effect of the H2S content on the relative permeability curves. This may be due to the limited availability of the relative permeability and capillary pressure data for acid gas/brine/rock systems; thus, more experimental measurements are required. (C) 2022 Institute of Rock and Soil Mechanics, Chinese Academy of Sciences. Production and hosting by Elsevier B.V. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
学科主题Engineering
语种英语
WOS记录号WOS:000891300600024
出版者SCIENCE PRESS
源URL[http://119.78.100.198/handle/2S6PX9GI/35314]  
专题中科院武汉岩土力学所
作者单位1.State Key Laboratory of Geomechanics and Geotechnical Engineering, Institute of Rock and Soil Mechanics, Chinese Academy of Sciences, Wuhan, 430071, China
2.University of Chinese Academy of Sciences, Beijing, 100049, China
3.Department of Engineering, Durham University, Durham, DH1 3LE, UK
4.Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou, 730000, China
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GB/T 7714
Zhang, Xiaoyan,Li, Qi,Simon, Mathias,et al. Effect of H2S content on relative permeability and capillary pressure characteristics of acid gas/brine/rock systems: A review[J]. JOURNAL OF ROCK MECHANICS AND GEOTECHNICAL ENGINEERING,2022,14(6):2003.
APA Zhang, Xiaoyan,Li, Qi,Simon, Mathias,Zheng, Guodong,&Tan, Yongsheng.(2022).Effect of H2S content on relative permeability and capillary pressure characteristics of acid gas/brine/rock systems: A review.JOURNAL OF ROCK MECHANICS AND GEOTECHNICAL ENGINEERING,14(6),2003.
MLA Zhang, Xiaoyan,et al."Effect of H2S content on relative permeability and capillary pressure characteristics of acid gas/brine/rock systems: A review".JOURNAL OF ROCK MECHANICS AND GEOTECHNICAL ENGINEERING 14.6(2022):2003.

入库方式: OAI收割

来源:武汉岩土力学研究所

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