中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Microwave-assisted catalytic pyrolysis of refuse-derived fuel (RDF) to improve pyrolysis performance and biochar properties

文献类型:期刊论文

作者Yang, Pu2; Jia, Dening2,3; Lin, Bingcheng2,4; Zhuang, Xiuzheng1,2; Bi, Xiaotao2,5
刊名FUEL PROCESSING TECHNOLOGY
出版日期2022-03-01
卷号227页码:11
关键词RDF Microwave catalytic pyrolysis K2CO3 Synergistic effect Biochar Specific surface area
ISSN号0378-3820
DOI10.1016/j.fuproc.2021.107129
通讯作者Bi, Xiaotao(tony.bi@ubc.ca)
英文摘要This paper investigated the feasibility of microwave-assisted catalytic pyrolysis (MACP) of refuse-derived fuel (RDF) to produce high quality biochar for the first time. Two main catalysts, K2CO3 and K3PO4, and their combination with bentonite or clinoptilolite were selected to mix with RDF in a fixed bed reactor exposed to microwave radiation. By comparing heating rate and biochar properties, the promising catalyst was identified as 20 wt% K2CO3 + 10 wt% bentonite due to its high heating rate (163 degrees C/min) and large specific surface area (264 m(2)/g) of biochar obtained under relatively low temperature (500 degrees C) and short microwave radiation time (30 min), much higher than previously reported values of RDF derived biochar (6-25 m(2)/g). K2CO3 showed higher heating rate and larger specific surface area of biochar than that of K3PO4 due to its prominent activation effect. Synergistic effect was observed when bentonite or clinoptilolite was added into K3PO4 which significantly improved microwave heating rate. Biochar produced from K2CO3 acts as a potential sorbent for retaining heavy metals in the biochar and soil due to its better porosity, while K3PO4 remaining in the biochar serves as essential nutrients for plant growth.
WOS关键词ACTIVATED CARBONS ; CONVENTIONAL PYROLYSIS ; ADSORPTIVE PROPERTIES ; SEWAGE-SLUDGE ; BIO-OIL ; POTASSIUM ; TEMPERATURE ; BIOMASS ; GASIFICATION ; WASTE
资助项目Natural Science and Engineering Research Council (NSERC) of Canada
WOS研究方向Chemistry ; Energy & Fuels ; Engineering
语种英语
WOS记录号WOS:000749962800001
出版者ELSEVIER
资助机构Natural Science and Engineering Research Council (NSERC) of Canada
源URL[http://ir.giec.ac.cn/handle/344007/35848]  
专题中国科学院广州能源研究所
通讯作者Bi, Xiaotao
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangdong Key Lab New & Renewable Energy Res & De, Guangzhou 510640, Peoples R China
2.Univ British Columbia, Dept Chem & Biol Engn, Vancouver, BC V6T 1Z3, Canada
3.Canadian Nucl Labs, 286 Plant Rd, Chalk River, ON K0J 1J0, Canada
4.UCAS, Hangzhou Inst Adv Study, Sch Environm, Hangzhou 310024, Peoples R China
5.Univ British Columbia, Clean Energy Res Ctr, 2360 East Mall, Vancouver, BC V6T 1Z3, Canada
推荐引用方式
GB/T 7714
Yang, Pu,Jia, Dening,Lin, Bingcheng,et al. Microwave-assisted catalytic pyrolysis of refuse-derived fuel (RDF) to improve pyrolysis performance and biochar properties[J]. FUEL PROCESSING TECHNOLOGY,2022,227:11.
APA Yang, Pu,Jia, Dening,Lin, Bingcheng,Zhuang, Xiuzheng,&Bi, Xiaotao.(2022).Microwave-assisted catalytic pyrolysis of refuse-derived fuel (RDF) to improve pyrolysis performance and biochar properties.FUEL PROCESSING TECHNOLOGY,227,11.
MLA Yang, Pu,et al."Microwave-assisted catalytic pyrolysis of refuse-derived fuel (RDF) to improve pyrolysis performance and biochar properties".FUEL PROCESSING TECHNOLOGY 227(2022):11.

入库方式: OAI收割

来源:广州能源研究所

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