Blue-Emitting InP/GaP/ZnS Quantum Dots with Enhanced Stability by Siloxane Capping: Implication for Electroluminescent Devices
文献类型：期刊论文
| 作者 | Shen, Cong3,4; Tao, Houng1; Zhu, Yanqing3 ; Li, Jingling5; Zou, Jianhua1; Wang, Lei1; Liang, Jingqiu2; Xiao, Xiudi3; Xu, Xueqing3; Xu, Gang3
|
| 刊名 | ACS APPLIED NANO MATERIALS
 |
| 出版日期 | 2022-02-25 |
| 卷号 | 5期号:2页码:11 |
| 关键词 | InP quantum dots blue-emitting core/shell structure siloxane capping stability QLEDs |
| DOI | 10.1021/acsanm.1c04486 |
| 通讯作者 | Zhu, Yanqing(zhuyq@ms.giec.ac.cn) ; Xu, Xueqing(xuxq@ms.giec.ac.cn) |
| 英文摘要 | InP quantum dots (QDs) with low toxicity are an ideal alternative to Cd-based QDs. However, the optical properties and stability of blue-emitting InP QDs are far inferior to those of red and green QDs. In this work, we report the synthesis of highly fluorescent InP/GaP/ZnS core/shell/ shell QDs with an emission wavelength of 484 nm and photoluminescence quantum yield of 71%, along with a full width at half-maximum as narrow as 45 nm. In addition, we encapsulated the QDs with siloxane via specific ligand exchange and condensation reactions to improve their stability. The corresponding siloxane capping QD light-emitting device (QLED) shows a maximum luminance of 690 Cd m(-2), an external quantum efficiency of 0.09%, and a much longer lifetime than pristine QDs. As a result, these enable the siloxane capping QDs to achieve a much stronger storage stability and a longer QLED lifetime than pristine QDs. |
| WOS关键词 | SELF-ASSEMBLED MONOLAYERS ; SHELL ; NANOCRYSTALS ; CORE ; EFFICIENT ; EMISSION ; BRIGHT ; (3-MERCAPTOPROPYL)TRIMETHOXYSILANE ; STRATEGY ; ROBUST |
| 资助项目 | Science and Technology Planning Project of Guangzhou[202007020004] ; Science and Technology Planning Project of Guangzhou[201904010171] ; Key Project on Synergy Collaborative Innovation of Guangzhou City[201704030069] ; Project on the Collaborative Innovation and Environmental Con-struction Platform of Guangdong Province[2018A050506067] ; Guangdong Basic and Applied Basic Research Foundation[2020A1515010544] ; Guangdong Basic and Applied Basic Research Foundation[2018A0303130146] ; Pearl River S&T Nova Program of Guangzhou[201806010090] ; National Natural Science Foundation of China[51902054] |
| WOS研究方向 | Science & Technology - Other Topics ; Materials Science |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000757912800001 |
| 资助机构 | Science and Technology Planning Project of Guangzhou ; Key Project on Synergy Collaborative Innovation of Guangzhou City ; Project on the Collaborative Innovation and Environmental Con-struction Platform of Guangdong Province ; Guangdong Basic and Applied Basic Research Foundation ; Pearl River S&T Nova Program of Guangzhou ; National Natural Science Foundation of China |
| 源URL | [http://ir.giec.ac.cn/handle/344007/35875]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zhu, Yanqing; Xu, Xueqing |
| 作者单位 | 1.Guangzhou New Vision Optoelect Technol Co Ltd, Guangzhou 510530, Peoples R China 2.Chinese Acad Sci, Changchun Inst Opt Fine Mech & Phys, Changchun 130033, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy Guangdong Prov, Key Lab New & Renewable Energy Res & Dev, Guangzhou 510640, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan 528000, Peoples R China |
| 推荐引用方式 GB/T 7714 | Shen, Cong,Tao, Houng,Zhu, Yanqing,et al. Blue-Emitting InP/GaP/ZnS Quantum Dots with Enhanced Stability by Siloxane Capping: Implication for Electroluminescent Devices[J]. ACS APPLIED NANO MATERIALS,2022,5(2):11. |
| APA | Shen, Cong.,Tao, Houng.,Zhu, Yanqing.,Li, Jingling.,Zou, Jianhua.,...&Xu, Gang.(2022).Blue-Emitting InP/GaP/ZnS Quantum Dots with Enhanced Stability by Siloxane Capping: Implication for Electroluminescent Devices.ACS APPLIED NANO MATERIALS,5(2),11. |
| MLA | Shen, Cong,et al."Blue-Emitting InP/GaP/ZnS Quantum Dots with Enhanced Stability by Siloxane Capping: Implication for Electroluminescent Devices".ACS APPLIED NANO MATERIALS 5.2(2022):11. |
入库方式： OAI收割
来源：广州能源研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。