Corncob pyrolysis: Improvement in hydrocarbon group types distribution of bio oil from co-catalysis over HZSM-5 and activated carbon
文献类型:期刊论文
作者 | Duan, Dengle1; Feng, Zhiqiang1; Zhang, Yongchuan1; Zhou, Tengyue1; Xu, Zhimin2; Wang, Qin1; Zhao, Yunfeng3; Wang, Chenguang4,5; Ruan, Roger6,7 |
刊名 | WASTE MANAGEMENT |
出版日期 | 2022-03-15 |
卷号 | 141页码:8-15 |
ISSN号 | 0956-053X |
关键词 | HZSM-5 Activated carbon Corncob Aromatics Co-catalytic pyrolysis |
DOI | 10.1016/j.wasman.2022.01.028 |
通讯作者 | Xu, Zhimin(xuzhiminjnu@sina.com) ; Zhao, Yunfeng(405685129@qq.com) |
英文摘要 | Zeolite and activated carbon (AC) have been demonstrated as promising and facile catalysts in degrading biomass into high-value added chemicals and bio-fuels, while the effects of combining zeolite and AC on the catalytic degradation of biomass have not been well understood. Here, co-catalytic pyrolysis of corncob over HZSM-5 and AC to produce aromatic-rich bio-oils was investigated for the first time. The effects of HZSM-5/AC ratio, pyrolysis temperature and catalyst/corncob ratio on products yields and components were explored. The optimal conversion condition was HZSM-5/AC ratio of 2:1, pyrolysis temperature of 500 celcius and catalyst/corncob ratio of 1:1. Up to 97.47% of the obtained bio-oil chemicals were jet-fuel ranged hydrocarbons, in which the selectivity of aromatics was 96.56%. The results revealed the existence of synergistic effect between HZSM-5 and AC. The present work suggested an economical and novel pathway to produce transportation jet fuel to ultimately expand the biomass application. |
WOS关键词 | MICROWAVE-ASSISTED PYROLYSIS ; LOW-DENSITY POLYETHYLENE ; LIGNOCELLULOSIC BIOMASS ; IN-SITU ; CONVERSION ; AROMATICS ; CHEMICALS ; VAPORS ; LIGNIN ; WASTE |
资助项目 | National Natural Science of China[E129kf0401] ; CAS Key Laboratory of Renewable Energy ; College Student Innovation Fund Project of Zhongkai University of Agriculture and Engineering ; High-level Introduction of Talent Scientific Research Start-up Fund of Zhongkai University of Agriculture and Engineering |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
WOS记录号 | WOS:000784289000002 |
资助机构 | National Natural Science of China ; CAS Key Laboratory of Renewable Energy ; College Student Innovation Fund Project of Zhongkai University of Agriculture and Engineering ; High-level Introduction of Talent Scientific Research Start-up Fund of Zhongkai University of Agriculture and Engineering |
源URL | [http://ir.giec.ac.cn/handle/344007/36170] |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Xu, Zhimin; Zhao, Yunfeng |
作者单位 | 1.Zhongkai Univ Agr & Engn, Guangdong Prov Key Lab Lingnan Specialty Food Sci, Guangzhou 510225, Peoples R China 2.Zhongkai Univ Agr & Engn, Coll Resources & Environm, Guangzhou 510225, Peoples R China 3.Shihezi Univ, Sch Food Sci & Technol, North Fourth Rd, Shihezi 832003, Peoples R China 4.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 5.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 6.Univ Minnesota, Ctr Biorefining, 1390 Eckles Ave, St Paul, MN 55108 USA 7.Univ Minnesota, Dept Bioprod & Biosyst Engn, 1390 Eckles Ave, St Paul, MN 55108 USA |
推荐引用方式 GB/T 7714 | Duan, Dengle,Feng, Zhiqiang,Zhang, Yongchuan,et al. Corncob pyrolysis: Improvement in hydrocarbon group types distribution of bio oil from co-catalysis over HZSM-5 and activated carbon[J]. WASTE MANAGEMENT,2022,141:8-15. |
APA | Duan, Dengle.,Feng, Zhiqiang.,Zhang, Yongchuan.,Zhou, Tengyue.,Xu, Zhimin.,...&Ruan, Roger.(2022).Corncob pyrolysis: Improvement in hydrocarbon group types distribution of bio oil from co-catalysis over HZSM-5 and activated carbon.WASTE MANAGEMENT,141,8-15. |
MLA | Duan, Dengle,et al."Corncob pyrolysis: Improvement in hydrocarbon group types distribution of bio oil from co-catalysis over HZSM-5 and activated carbon".WASTE MANAGEMENT 141(2022):8-15. |
入库方式: OAI收割
来源:广州能源研究所
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