中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support

文献类型:期刊论文

作者Luo, Fengying1,2; Wang, Zeyu1,2; Li, Xiangnan1; Lang, Lin1; Li, Xinjun1; Yin, Xiuli1
刊名NEW JOURNAL OF CHEMISTRY
出版日期2022-05-16
卷号46期号:19页码:9304-9311
ISSN号1144-0546
DOI10.1039/d1nj06013a
通讯作者Li, Xinjun() ; Yin, Xiuli()
英文摘要Highly dispersed Ni-based catalysts were derived from self-reconstruction of the LaNiO3 perovskite, which were prepared via the sol-gel process. Activity measurements indicated that the as-prepared catalysts exhibit an excellent dry methane reforming catalytic performance, which can achieve CH4 conversion of 84.17% and 83.35% at 650 degrees C at a gas hourly space velocity (GHSV) of 128 L (g(cat) h)(-1). The physicochemical characterization of the as-prepared catalysts suggested that the transition layer of La2NiO4 is formed between metallic Ni-0 and the La(OH)(3) support. The Ni-0-Ni2+ dipole on the support is relevant to the catalytic activity for the dry methane reforming reaction.
WOS关键词RAY PHOTOELECTRON-SPECTROSCOPY ; SYNGAS PRODUCTION ; OXIDE CATALYSTS ; CARBON-DIOXIDE ; PERFORMANCE ; CH4 ; REDUCTION ; NI/LA2O3
资助项目National Key R&D Program of China[2019YFB1503902] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA21060600] ; Science and Technology Program of Guangzhou[202002030126]
WOS研究方向Chemistry
语种英语
出版者ROYAL SOC CHEMISTRY
WOS记录号WOS:000788237400001
资助机构National Key R&D Program of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Science and Technology Program of Guangzhou
源URL[http://ir.giec.ac.cn/handle/344007/36297]  
专题中国科学院广州能源研究所
通讯作者Li, Xinjun; Yin, Xiuli
作者单位1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Luo, Fengying,Wang, Zeyu,Li, Xiangnan,et al. Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support[J]. NEW JOURNAL OF CHEMISTRY,2022,46(19):9304-9311.
APA Luo, Fengying,Wang, Zeyu,Li, Xiangnan,Lang, Lin,Li, Xinjun,&Yin, Xiuli.(2022).Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support.NEW JOURNAL OF CHEMISTRY,46(19),9304-9311.
MLA Luo, Fengying,et al."Highly dispersed Ni-based catalysts derived from the LaNiO3 perovskite for dry methane reforming: promotional effect of the Ni-0-Ni2+ dipole inlaid on the support".NEW JOURNAL OF CHEMISTRY 46.19(2022):9304-9311.

入库方式: OAI收割

来源:广州能源研究所

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