Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production
文献类型：期刊论文
| 作者 | Wang, Shuxiao1,2,3,4; Zhang, Yuyuan6; Shan, Rui1,2,3,5; Gu, Jing1,2,3,5; Yuan, Haoran1,2,3,5 ; Chen, Yong1,2,3,4,5
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| 刊名 | ENERGY
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| 出版日期 | 2022-05-01 |
| 卷号 | 246页码:9 |
| ISSN号 | 0360-5442 |
| 关键词 | Thermochemical Catalytic reforming Syngas Tar removal Hydrogen Pyrolysis char |
| DOI | 10.1016/j.energy.2022.123342 |
| 通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
| 英文摘要 | The removal of biomass tar is the key technology in the pyrolysis and gasification technology, and the advantages of solid waste pyrolysis char in tar removal gradually become prominent. In this paper, the tar model compound (benzene) was catalytic reformed by a novel hybrid carrier catalysts using a laboratory dual-stage reactor. The hybrid carrier catalyst was prepared by wet impregnation method with nickel active substance, and the carrier was a two-material mixture of peat char and sludge char. In the reaction of steam reforming benzene, the effects of temperature (600-800 degrees C) and nickel load (5%-20%) on benzene conversion were investigated, showing that the catalyst have good benzene removal ability (91.8%) and the gas product with high syngas content (93.6%) was obtained. The surface properties of the catalyst was detected by SEM, EDS, BET and XRD detection, in order to prove that the catalytic performance was related to surface nanoparticles and abundant active sites. The novel hybrid carrier catalyst can effectively remove the aromatic tar and produce syngas with high performance. (c) 2022 Elsevier Ltd. All rights reserved. |
| WOS关键词 | MICROWAVE PYROLYSIS ; BOTTOM ASH ; RICE HUSK ; CRACKING ; GASIFICATION ; TOLUENE ; SLUDGE ; CARBON ; DECOMPOSITION ; CONVERSION |
| 资助项目 | National Key R&D Pro-gram of China[2018YFC1901200] ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; National Natural Science Foundation of China[51906248] ; National Natural Science Foundation of China[51906045] ; CAS Key Laboratory of Renewable Energy[E029040101] ; Guangdong Province Science and Technology Planning Project[2019B110210003] |
| WOS研究方向 | Thermodynamics ; Energy & Fuels |
| 语种 | 英语 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| WOS记录号 | WOS:000791830300004 |
| 资助机构 | National Key R&D Pro-gram of China ; Key Special Project for Intro-duced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; National Natural Science Foundation of China ; CAS Key Laboratory of Renewable Energy ; Guangdong Province Science and Technology Planning Project |
| 源URL | [http://ir.giec.ac.cn/handle/344007/36379]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yuan, Haoran |
| 作者单位 | 1.Chinese Acad Sci, Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 4.Nanjing Tech Univ, Nanjing 211816, Peoples R China 5.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China 6.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,et al. Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production[J]. ENERGY,2022,246:9. |
| APA | Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,Gu, Jing,Yuan, Haoran,&Chen, Yong.(2022).Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production.ENERGY,246,9. |
| MLA | Wang, Shuxiao,et al."Steam reforming of biomass tar model compound over two waste char-based Ni catalysts for syngas production".ENERGY 246(2022):9. |
入库方式： OAI收割
来源：广州能源研究所
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