High-yield H-2 production from polypropylene through pyrolysis-catalytic reforming over activated carbon based nickel catalyst
文献类型：期刊论文
| 作者 | Wang, Shuxiao1,2,4,5; Zhang, Yuyuan6; Shan, Rui1,3,4; Gu, Jing1,3,4; Huhe, Taoli2,7; Ling, Xiang2; Yuan, Haoran1,3,4 ; Chen, Yong1,2,3,4
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| 刊名 | JOURNAL OF CLEANER PRODUCTION
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| 出版日期 | 2022-06-10 |
| 卷号 | 352页码:12 |
| 关键词 | Pyrolysis Catalytic reforming Plastic H-2 production Ni catalyst |
| ISSN号 | 0959-6526 |
| DOI | 10.1016/j.jclepro.2022.131566 |
| 通讯作者 | Yuan, Haoran(yuanhr@ms.giec.ac.cn) |
| 英文摘要 | With the aggravation of energy crisis and environmental pollution, green and renewable new alternative energy has become the focus of global attention. Hydrogen energy has become an important part of the global energy pattern in the future. Conversion of solid waste plastics into hydrogen energy by pyrolysis/gasification is a promising solution. This study aims to explore a method of high-yield in hydrogen by breaking down polypropylene, a cheap and efficient nickel catalyst is prepared and applied to the experimental study of hydrogen production by pyrolysis-catalytic reforming. The effects of catalytic temperature, Ni loading (%) and catalyst addition amount on hydrogen production of catalyst were investigated, the hydrogen production was increased by introducing water vapor. Under the optimized reaction parameters (catalytic temperature 900 ?C, PP to catalyst ratio 1:0.75, Ni loading 15 wt%), the hydrogen yield is up to 40.24 mmol/gPP without water and 134.91 mmol/gPP with water, the addition of water significantly increased hydrogen production. this results have obvious advantages in hydrogen production compared with similar studies. Furthermore, the existence of various forms (snake-like, straight carbon nanotubes and carbon nanospheres) of carbon deposition found in this paper can provide new ideas for researchers working on graphite carbon. This study provides an effective new approaches for enhancing hydrogen production by pyrolysis/gasification of waste plastics. |
| WOS关键词 | TAR MODEL COMPOUNDS ; HYDROGEN-PRODUCTION ; PLASTIC WASTE ; GASIFICATION ; DECOMPOSITION ; NANOTUBES ; NI ; BIOMASS ; COPRODUCTION ; TEMPERATURE |
| 资助项目 | National Key R&D Program of China[2018YFC1901200] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Labo-ratory (Guangzhou)[GML2019ZD0101] ; National Natural Science Foundation of China[51906248] ; National Natural Science Foundation of China[51906045] |
| WOS研究方向 | Science & Technology - Other Topics ; Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000793422700004 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | National Key R&D Program of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Labo-ratory (Guangzhou) ; National Natural Science Foundation of China |
| 源URL | [http://ir.giec.ac.cn/handle/344007/36439]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Yuan, Haoran |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, 2 Nengyuan Rd, Guangzhou 510640, Guangdong, Peoples R China 2.Nanjing Tech Univ, Nanjing 211816, Peoples R China 3.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China 4.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 5.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 6.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan, Peoples R China 7.Changzhou Univ, Changzhou, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Shuxiao,Zhang, Yuyuan,Shan, Rui,et al. High-yield H-2 production from polypropylene through pyrolysis-catalytic reforming over activated carbon based nickel catalyst[J]. JOURNAL OF CLEANER PRODUCTION,2022,352:12. |
| APA | Wang, Shuxiao.,Zhang, Yuyuan.,Shan, Rui.,Gu, Jing.,Huhe, Taoli.,...&Chen, Yong.(2022).High-yield H-2 production from polypropylene through pyrolysis-catalytic reforming over activated carbon based nickel catalyst.JOURNAL OF CLEANER PRODUCTION,352,12. |
| MLA | Wang, Shuxiao,et al."High-yield H-2 production from polypropylene through pyrolysis-catalytic reforming over activated carbon based nickel catalyst".JOURNAL OF CLEANER PRODUCTION 352(2022):12. |
入库方式： OAI收割
来源：广州能源研究所
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