中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Influence of cold-seep environments on the kinetics of methane hydrate formation

文献类型:期刊论文

作者Zhang, Yitong1,3,4,6; Xi, Shichuan1,6; Du, Zengfeng1,3,4,6; Luan, Zhendong1,3,4,6; Zhang, Xin1,2,3,4,5,6
刊名MARINE AND PETROLEUM GEOLOGY
出版日期2023-09-01
卷号155页码:9
ISSN号0264-8172
关键词Methane hydrate Cold seep environment In situ Raman spectroscopy Hydrate formation
DOI10.1016/j.marpetgeo.2023.106401
通讯作者Zhang, Xin(xzhang@qdio.ac.cn)
英文摘要Methane hydrate (MH) is widely distributed in active deep-sea cold-seep areas. The complex environment of cold seeps influences MH formation. Investigating the effects of cold-seep environments on MH formation can provide an in-depth understanding of the formation mechanism of MH and kinetic process of cold-seep development and evolution. In this study, multiple MH formation experiments were conducted in the laboratory to investigate the effects of a cold-seep environment on the kinetics of hydrate formation. Considering the cold-seep fluid and bottom seawater as the samples, MH was formed in the capillary under the same pressure-temperature conditions as those in cold-seep environments. The entire process of MH formation was recorded by time-series Raman spectra and video, and the results demonstrated the promotion of MH formation by solid particles, especially authigenic carbonates. Compared to 20 min in seawater, the induction time of 2 min in cold-seep fluids indicated promotion of hydrate formation by tiny particles and by its lower salinity. Notably, the reduction in salinity in the cold-seep fluid may be attributed to the dilution effect of pure water produced by hydrate decomposition, indicating the presence of a hydrate memory effect. Overall, our results are in agreement with those of the in situ hydrate formation experiment in a cold-seep environment. A model of hydrate formation in a cold-seep environment has been proposed, which can aid in understanding the kinetics of hydrate formation.
WOS关键词IN-SITU RAMAN ; AUTHIGENIC CARBONATES ; GAS HYDRATE ; FORMOSA RIDGE ; SEA-FLOOR ; DISSOCIATION ; PHASE ; WATER
资助项目National Natural Science Foundation of China[92058206] ; National Natural Science Foundation of China[52001303] ; National Natural Science Foundation of China[42221005] ; Strategic Priority Research Program, CAS[XDB42040302] ; Young Taishan Scholars Program[tsqn201909158] ; Key Project of Ocean Research Center, Chinese Academy of Sciences[COMS2020J03]
WOS研究方向Geology
语种英语
出版者ELSEVIER SCI LTD
WOS记录号WOS:001041851900001
源URL[http://ir.qdio.ac.cn/handle/337002/182680]  
专题海洋研究所_海洋地质与环境重点实验室
海洋研究所_深海极端环境与生命过程研究中心
通讯作者Zhang, Xin
作者单位1.Chinese Acad Sci, Key Lab Marine Geol & Environm, Qingdao 266071, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Inst Oceanol, Ctr Deep Sea Res, Qingdao 266071, Peoples R China
4.Chinese Acad Sci, CAS Key Lab Marine Geol & Environm, Qingdao 266071, Peoples R China
5.Lab Marine Geol, LaoShan Lab, Qingdao 266061, Peoples R China
6.Chinese Acad Sci, Inst Oceanol, Ctr Deep Sea Res, Ctr Ocean Mega Sci, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Yitong,Xi, Shichuan,Du, Zengfeng,et al. Influence of cold-seep environments on the kinetics of methane hydrate formation[J]. MARINE AND PETROLEUM GEOLOGY,2023,155:9.
APA Zhang, Yitong,Xi, Shichuan,Du, Zengfeng,Luan, Zhendong,&Zhang, Xin.(2023).Influence of cold-seep environments on the kinetics of methane hydrate formation.MARINE AND PETROLEUM GEOLOGY,155,9.
MLA Zhang, Yitong,et al."Influence of cold-seep environments on the kinetics of methane hydrate formation".MARINE AND PETROLEUM GEOLOGY 155(2023):9.

入库方式: OAI收割

来源:海洋研究所

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