A solar-driven degradation-evaporation strategy for membrane self-cleaning in the efficient separation of viscous crude oil/ water emulsions
文献类型：期刊论文
| 作者 | Yu, Jiacheng2; Cao, Changqian2; Pan, Yongxin1,2 |
| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2023-09-05 |
| 卷号 | 457页码:12 |
| ISSN号 | 0304-3894 |
| 关键词 | Wastewater treatment Anti-crude-oil-fouling Self-cleaning membrane Photo-Fenton Solar-driven evaporation |
| DOI | 10.1016/j.jhazmat.2023.131826 |
| 英文摘要 | Membrane separation techniques are promising methods for effectively treating hazardous emulsified oily wastewater, but membrane fouling remains a serious challenge because the high viscosity and complex composition of crude oil make it easy to adhere to membranes and difficult to be removed by conventional physical or chemical cleaning means. Herein, a two-stage solar-driven (photo-Fenton degradation/evaporation) strategy was proposed to realize the self-cleaning of membranes fouled by viscous crude oil (>60,000 mPa s), wherein the photo-Fenton process helped to degrade the heavy components into light components, and all light components removed during the solar-driven evaporation process. A 1D/2D heterostructure membrane with photo-Fenton activity and anti-crude-oil-fouling performance was prepared via a facile self-assembly vacuumassist method. The addition of rod-like g-C3N4 (RCN) increased the interlayer distance of alpha-FeOOH/porous gC3N4 (FPCN) nanosheets, resulting in a high permeation flux. The FPCN-RCN membrane exhibited both high permeation flux of 779 +/- 19 L m(-2)h(-1)bar(-1) and a separation efficiency of 99.4% for highly viscous crude oil-inwater emulsion. Importantly, the viscous crude oil fouled on the membrane was completely removed by the photo-Fenton degradation/solar-driven evaporation strategy, and the flux recovery rate of the membrane was similar to 100%. Therefore, the FPCN-RCN membrane combined with the novel self-cleaning strategy exhibits great potential for practical emulsified oily wastewater treatment. |
| WOS关键词 | GRAPHITIC CARBON NITRIDE ; G-C3N4 ; NANOSHEETS |
| 资助项目 | National Natural Science Foundation of China[42204083] ; National Natural Science Foundation of China[41621004] ; China Postdoctoral Science Foundation Funded Project[2022M713127] ; PetroChina Innovation Foundation[2020D-5007-0105] ; Key Research Program of the Institute of Geology amp; Geophysics, CAS[IGGCAS-201903] ; Key Research Program of the Institute of Geology amp; Geophysics, CAS[IGGCAS-202201] |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| 出版者 | ELSEVIER |
| WOS记录号 | WOS:001023543200001 |
| 资助机构 | National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; China Postdoctoral Science Foundation Funded Project ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; PetroChina Innovation Foundation ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS ; Key Research Program of the Institute of Geology amp; Geophysics, CAS |
| 源URL | [http://ir.iggcas.ac.cn/handle/132A11/111310]  |
| 专题 | 地质与地球物理研究所_中国科学院地球与行星物理重点实验室 |
| 通讯作者 | Yu, Jiacheng; Cao, Changqian |
| 作者单位 | 1.Univ Chinese Acad Sci, Coll Earth Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Inst Geol & Geophys, Innovat Acad Earth Sci, Key Lab Earth & Planetary Phys, Beijing 100029, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yu, Jiacheng,Cao, Changqian,Pan, Yongxin. A solar-driven degradation-evaporation strategy for membrane self-cleaning in the efficient separation of viscous crude oil/ water emulsions[J]. JOURNAL OF HAZARDOUS MATERIALS,2023,457:12. |
| APA | Yu, Jiacheng,Cao, Changqian,&Pan, Yongxin.(2023).A solar-driven degradation-evaporation strategy for membrane self-cleaning in the efficient separation of viscous crude oil/ water emulsions.JOURNAL OF HAZARDOUS MATERIALS,457,12. |
| MLA | Yu, Jiacheng,et al."A solar-driven degradation-evaporation strategy for membrane self-cleaning in the efficient separation of viscous crude oil/ water emulsions".JOURNAL OF HAZARDOUS MATERIALS 457(2023):12. |
入库方式： OAI收割
来源：地质与地球物理研究所
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