Portable smartphone-assisted highly sensitive detection of mercury ions based on gold nanoparticle-modified NH2-UiO-66 metal-organic framework
文献类型：期刊论文
| 作者 | Wang, Shasha4; Wang, Yifei4; Ma, Jiping4; Huang, Chaonan4; Chen, Lingxin1,2,3
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| 刊名 | ANALYTICAL AND BIOANALYTICAL CHEMISTRY
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| 出版日期 | 2023-12-15 |
| 页码 | 10 |
| ISSN号 | 1618-2642 |
| 关键词 | Gold nanoparticles Metal-organic framework Mercury ions RGB analysis Smartphone-assisted detection |
| DOI | 10.1007/s00216-023-05090-y |
| 通讯作者 | Ma, Jiping(majiping@qut.edu.cn) ; Chen, Lingxin(lxchen@yic.ac.cn) |
| 英文摘要 | A novel portable smartphone-assisted colorimetric method was reported for the determination of Hg2+ with good analytical performance. A Zr(IV)-based metal-organic framework functionalized with amino groups (NH2-UiO-66) has been adopted as a supporting platform to anchor gold nanoparticles (AuNPs), avoiding the migration and aggregation of AuNPs. With the addition of Hg2+, the formation of gold amalgam proved possible to enhance peroxidase-like activity of the composite (AuNPs/NH2-UiO-66), accelerating the oxidization of zymolyte 3,3 ',5,5 '-tetramethylbenzidine (TMB). In the meantime, the color of the reaction solution turned a vivid blue, and the red, green, and blue (RGB) values of the solution color changed accordingly. On account of this strategy, the quantitative detection of Hg2+ could be achieved. After the optimization of the experiment conditions, the average color intensity (I-c) resulting from RGB values was linear related to the concentration of Hg2+ from 10 to 100 nM, accompanied with a detection limit (LOD) down to 5.4 nM calculated by 3 sigma/S. The successful application of the designed method has been promoted to detect Hg2+ in some water samples, displaying a great potential in practical application. Furthermore, the use of a smartphone made our proposed method simple and accurate, and thus puts forward a possible way for in situ and real-time monitoring. |
| WOS关键词 | COLORIMETRIC DETECTION ; AQUEOUS-SOLUTION ; SPECIATION ; UIO-66-NH2 ; EXTRACTION ; SAMPLES ; HG(II) ; SENSOR ; WATER ; HG2+ |
| WOS研究方向 | Biochemistry & Molecular Biology ; Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:001125113600001 |
| 资助机构 | National Natural Science Foundation of China ; Shandong Provincial Natural Science Foundation |
| 源URL | [http://ir.yic.ac.cn/handle/133337/33147]  |
| 专题 | 烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室 烟台海岸带研究所_山东省海岸带环境工程技术研究中心 |
| 通讯作者 | Ma, Jiping; Chen, Lingxin |
| 作者单位 | 1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn & Technol,Shandong K, CAS Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China 2.Binzhou Med Univ, Sch Pharm, Yantai 264003, Peoples R China 3.Shaoxing Univ, Coll Chem & Chem Engn, Shaoxing 312000, Peoples R China 4.Qingdao Univ Technol, Sch Environm & Municipal Engn, Qingdao 266520, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Shasha,Wang, Yifei,Ma, Jiping,et al. Portable smartphone-assisted highly sensitive detection of mercury ions based on gold nanoparticle-modified NH2-UiO-66 metal-organic framework[J]. ANALYTICAL AND BIOANALYTICAL CHEMISTRY,2023:10. |
| APA | Wang, Shasha,Wang, Yifei,Ma, Jiping,Huang, Chaonan,&Chen, Lingxin.(2023).Portable smartphone-assisted highly sensitive detection of mercury ions based on gold nanoparticle-modified NH2-UiO-66 metal-organic framework.ANALYTICAL AND BIOANALYTICAL CHEMISTRY,10. |
| MLA | Wang, Shasha,et al."Portable smartphone-assisted highly sensitive detection of mercury ions based on gold nanoparticle-modified NH2-UiO-66 metal-organic framework".ANALYTICAL AND BIOANALYTICAL CHEMISTRY (2023):10. |
入库方式： OAI收割
来源：烟台海岸带研究所
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