中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 烟台海岸带研究所
  3. 中国科学院烟台海岸带研究所
  4. 中科院海岸带环境过程与生态修复重点实验室
Spatiotemporal distribution and particle-water partitioning of polycyclic aromatic hydrocarbons in Bohai Sea, China

文献类型：期刊论文

作者Chen, Chongtai1; Lin, Tian1; Sun, Xu3; Wu, Zilan2; Tang, Jianhui3
刊名WATER RESEARCH
出版日期2023-10-01
卷号244页码:9
ISSN号0043-1354
关键词PAHs Spatiotemporal distribution Rainy season Bohai sea Particle-water partitioning
DOI10.1016/j.watres.2023.120440
通讯作者Lin, Tian(lintian@vip.gyig.ac.cn) ; Tang, Jianhui(jhtang@yic.ac.cn)
英文摘要The Bohai Sea is one of the most polluted marine areas in China with polycyclic aromatic hydrocarbons (PAHs) due to its unique hydrological and geographical environment. To investigate differences in PAH concentrations, composition, and particle-water partitioning before and after the rainy reason, water samples were collected during two surveying voyages covering most of the area of the Bohai Sea. Total and dissolved PAH concentrations were higher during the June voyage (total PAHs: 32.29 & PLUSMN; 15.18 ng/L, dissolved PAHs: 31.25 & PLUSMN; 15.26 ng/L) than the August voyage (total PAHs: 15.98 & PLUSMN; 6.39 ng/L, dissolved PAHs: 11.21 & PLUSMN; 5.59 ng/L). The opposite trend was observed for particulate PAHs (June: 1.04 & PLUSMN; 1.01 ng/L, August: 4.78 & PLUSMN; 2.96 ng/L). Among particulate PAHs, an unusually high proportion (65.07%) of low-molecular-weight (LMW) PAHs was observed during the August voyage, which was significantly higher than the proportion during the June voyage (21.86%). This high proportion was inconsistent with the general distribution of PAHs in the aquatic environment according to their physicochemical properties. The excess LMW PAHs adsorbed on suspended particulate matter arose mainly from soil affected by the petrochemical industry of the Bohai Economic Rim, and were carried with particles on runoff into the Bohai Sea during the rainy season. An estimated 5.49 t of LMW PAHs transitioned from the particulate phase to the dissolved phase during the rainy season. This transfer of LMW PAHs from coastal soil to the water column may be an important source of PAHs in the Bohai Sea.
WOS关键词ECOLOGICAL RISK-ASSESSMENT ; SUSPENDED PARTICULATE MATTER ; SOURCE APPORTIONMENT ; SEASONAL-VARIATIONS ; SURFACE SEDIMENTS ; FOOD-WEB ; PAHS ; RIVER ; SEAWATER ; EXCHANGE
WOS研究方向Engineering ; Environmental Sciences & Ecology ; Water Resources
语种英语
WOS记录号WOS:001060516900001
资助机构Joint Funds of the National Natural Science Foundation of China ; National Natural Science Foundation of China (Youth Program)
源URL[http://ir.yic.ac.cn/handle/133337/33507]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_近岸生态与环境实验室
通讯作者Lin, Tian; Tang, Jianhui
作者单位1.Shanghai Ocean Univ, Coll Marine Ecol & Environm, Shanghai 201306, Peoples R China
2.Natl Marine Environm Monitoring Ctr, China State Environm Protect Key Lab Coastal Ecosy, Dalian 116023, Peoples R China
3.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714		 Chen, Chongtai,Lin, Tian,Sun, Xu,et al. Spatiotemporal distribution and particle-water partitioning of polycyclic aromatic hydrocarbons in Bohai Sea, China[J]. WATER RESEARCH,2023,244:9.
APA Chen, Chongtai,Lin, Tian,Sun, Xu,Wu, Zilan,&Tang, Jianhui.(2023).Spatiotemporal distribution and particle-water partitioning of polycyclic aromatic hydrocarbons in Bohai Sea, China.WATER RESEARCH,244,9.
MLA Chen, Chongtai,et al."Spatiotemporal distribution and particle-water partitioning of polycyclic aromatic hydrocarbons in Bohai Sea, China".WATER RESEARCH 244(2023):9.

入库方式： OAI收割

来源：烟台海岸带研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。