Polarized Raman scattering and magnetic ordering in Mn lightly doped van der Waals Cr1-xMnxGeTe3 crystals
文献类型:期刊论文
作者 | Xie, Qiyun5,6; Zeng, Shuai5,6; Chen, Yalong5,6; Chen, Limin5,6; Wang, Wei3,4; Ma, Ligang2; Cheng, Guofeng1 |
刊名 | APPLIED PHYSICS LETTERS |
出版日期 | 2024-02-05 |
卷号 | 124期号:6页码:8 |
ISSN号 | 0003-6951 |
DOI | 10.1063/5.0186428 |
通讯作者 | Wang, Wei(iamwwang@njtech.edu.cn) ; Cheng, Guofeng(gfcheng@mail.sic.ac.cn) |
英文摘要 | A layered van der Waals ferromagnet CrGeTe3 has attracted considerable interest due to the great potential for exploring low-power functional spintronic devices. However, research on the incorporation of chemical substitution in CrGeTe3 to tune the lattice vibrations and magnetic interactions is still lacking. In this work, an understanding of the phonon property and magnetic orders in Mn lightly doped Cr1-xMnxGeTe3 single crystals has been reported. It is found that the phonon symmetries are preserved over the studied Mn substitution content, as confirmed by angle-resolved polarized Raman spectroscopy and first-principles calculations. Furthermore, clear signatures of improved ferromagnetic Curie-Weiss temperature and magnetic moment are observed by detailed magnetic measurements. The higher magnetic moment of Mn ions, the variation of Mn-Te-Cr angle, Mn-induced hole doping, and the concomitant strain effect may all contribute to the enhanced ferromagnetism. Overall, our results demonstrate that chemical substitution is an effective pathway to engineering the lattice and magnetism of CrGeTe3. |
WOS关键词 | FERROMAGNETISM ; SPECTROSCOPY |
资助项目 | Natural Science Foundation of Nanjing University of Posts and Telecommunications ; Postgraduate Research & Practice Innovation Program of Jiangsu Province[SJCX22_0256] ; Postgraduate Research & Practice Innovation Program of Jiangsu Province[KYCX21_0708] ; [NY221063] ; [NY220186] |
WOS研究方向 | Physics |
语种 | 英语 |
出版者 | AIP Publishing |
WOS记录号 | WOS:001159087600006 |
源URL | [http://119.78.100.183/handle/2S10ELR8/309889] |
专题 | 中国科学院上海药物研究所 |
通讯作者 | Wang, Wei; Cheng, Guofeng |
作者单位 | 1.Chinese Acad Sci, Shanghai Inst Ceram, Anal & Testing Ctr Inorgan Mat, Shanghai 200050, Peoples R China 2.Nanjing Xiaozhuang Univ, Sch Elect Engn, Nanjing 211171, Peoples R China 3.Nanjing Tech Univ, Inst Adv Mat, Jiangsu Natl Synerget Innovat Ctr Adv Mat, Nanjing 211816, Peoples R China 4.Nanjing Tech Univ, Jiangsu Natl Synerget Innovat Ctr Adv Mat, Key Lab Flexible Elect, Nanjing 211816, Peoples R China 5.Nanjing Univ Posts & Telecommun, Coll Flexible Elect Future Technol, Nanjing 210023, Jiangsu, Peoples R China 6.Nanjing Univ Posts & Telecommun, Coll Elect & Opt Engn, Nanjing 210023, Jiangsu, Peoples R China |
推荐引用方式 GB/T 7714 | Xie, Qiyun,Zeng, Shuai,Chen, Yalong,et al. Polarized Raman scattering and magnetic ordering in Mn lightly doped van der Waals Cr1-xMnxGeTe3 crystals[J]. APPLIED PHYSICS LETTERS,2024,124(6):8. |
APA | Xie, Qiyun.,Zeng, Shuai.,Chen, Yalong.,Chen, Limin.,Wang, Wei.,...&Cheng, Guofeng.(2024).Polarized Raman scattering and magnetic ordering in Mn lightly doped van der Waals Cr1-xMnxGeTe3 crystals.APPLIED PHYSICS LETTERS,124(6),8. |
MLA | Xie, Qiyun,et al."Polarized Raman scattering and magnetic ordering in Mn lightly doped van der Waals Cr1-xMnxGeTe3 crystals".APPLIED PHYSICS LETTERS 124.6(2024):8. |
入库方式: OAI收割
来源:上海药物研究所
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