中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers

文献类型:期刊论文

作者Tong, Yali1; Gao, Jiajia1; Yue, Tao1,5; Yuan, Yue2; Tang, Yu3; Wang, Lingqing4
刊名JOURNAL OF HAZARDOUS MATERIALS
出版日期2024-03-15
卷号466页码:13
关键词Coal-fired industrial boilers (CFIBs) Heavy metals (HMs) Emission inventory Waste inventory Material flow
ISSN号0304-3894
DOI10.1016/j.jhazmat.2024.133678
通讯作者Yue, Tao(yuetao@ustb.edu.cn)
英文摘要Coal-fired industrial boilers (CFIBs) are critical anthropogenic contributors of heavy metals (HMs) because of their high coal consumption and complicated air pollution control facilities (APCDs). This study explored the flows of Hg, As, Cd, Cr, and Pb in CFIBs at regional scale by establishing a boiler-level HMs inflow-outflow inventory. The results indicate that large-capacity CFIBs (>= 65 t/h) are the leading contributors to HMs inflows. The inflow intensities of HMs in the provinces exhibited three classes of clustering characteristics. Significant regional heterogeneity was characterized by the distribution of HMs inflows and outflows, with higher HMs inflows and outflows in the northern and east-central coastal areas. However, the relatively low synergistic control efficiency of Cd in Northwest China resulted in a higher contribution of waste than inflow. The wastes generated during the operation of CFIBs are the major outflows of HMs. Hg was observed to have the highest outflow of atmospheric emissions owing to its high volatility. In addition, significant differences in the magnitude of HM outflow were identified among the provinces. The application of efficient APCDs contributes significantly to the partitioning of HMs into waste flows, thereby decreasing regional atmospheric emissions.
WOS关键词HAZARDOUS TRACE-ELEMENTS ; PRIMARY AIR-POLLUTANTS ; HEAVY-METALS ; POWER-PLANTS ; ELECTROSTATIC PRECIPITATOR ; MERCURY EMISSIONS ; FLY-ASH ; COMBUSTION ; BEHAVIOR ; SPECIATION
资助项目Beijing Natural Science Foundation[8192014] ; National Key Research and Development Program of China[2016YFC0208103]
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
WOS记录号WOS:001177560800001
出版者ELSEVIER
资助机构Beijing Natural Science Foundation ; National Key Research and Development Program of China
源URL[http://ir.igsnrr.ac.cn/handle/311030/203980]  
专题中国科学院地理科学与资源研究所
通讯作者Yue, Tao
作者单位1.Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China
2.Chinese Res Inst Environm Sci, Res Ctr Environm Pollut Control Engn Technol, Beijing 100012, Peoples R China
3.Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China
4.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China
5.Univ Sci & Technol Beijing, 30 Xueyuan Rd, Beijing 100083, Peoples R China
推荐引用方式
GB/T 7714
Tong, Yali,Gao, Jiajia,Yue, Tao,et al. Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers[J]. JOURNAL OF HAZARDOUS MATERIALS,2024,466:13.
APA Tong, Yali,Gao, Jiajia,Yue, Tao,Yuan, Yue,Tang, Yu,&Wang, Lingqing.(2024).Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers.JOURNAL OF HAZARDOUS MATERIALS,466,13.
MLA Tong, Yali,et al."Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers".JOURNAL OF HAZARDOUS MATERIALS 466(2024):13.

入库方式: OAI收割

来源:地理科学与资源研究所

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