Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers
文献类型:期刊论文
作者 | Tong, Yali1; Gao, Jiajia1; Yue, Tao1,5; Yuan, Yue2; Tang, Yu3; Wang, Lingqing4 |
刊名 | JOURNAL OF HAZARDOUS MATERIALS
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出版日期 | 2024-03-15 |
卷号 | 466页码:13 |
关键词 | Coal-fired industrial boilers (CFIBs) Heavy metals (HMs) Emission inventory Waste inventory Material flow |
ISSN号 | 0304-3894 |
DOI | 10.1016/j.jhazmat.2024.133678 |
通讯作者 | Yue, Tao(yuetao@ustb.edu.cn) |
英文摘要 | Coal-fired industrial boilers (CFIBs) are critical anthropogenic contributors of heavy metals (HMs) because of their high coal consumption and complicated air pollution control facilities (APCDs). This study explored the flows of Hg, As, Cd, Cr, and Pb in CFIBs at regional scale by establishing a boiler-level HMs inflow-outflow inventory. The results indicate that large-capacity CFIBs (>= 65 t/h) are the leading contributors to HMs inflows. The inflow intensities of HMs in the provinces exhibited three classes of clustering characteristics. Significant regional heterogeneity was characterized by the distribution of HMs inflows and outflows, with higher HMs inflows and outflows in the northern and east-central coastal areas. However, the relatively low synergistic control efficiency of Cd in Northwest China resulted in a higher contribution of waste than inflow. The wastes generated during the operation of CFIBs are the major outflows of HMs. Hg was observed to have the highest outflow of atmospheric emissions owing to its high volatility. In addition, significant differences in the magnitude of HM outflow were identified among the provinces. The application of efficient APCDs contributes significantly to the partitioning of HMs into waste flows, thereby decreasing regional atmospheric emissions. |
WOS关键词 | HAZARDOUS TRACE-ELEMENTS ; PRIMARY AIR-POLLUTANTS ; HEAVY-METALS ; POWER-PLANTS ; ELECTROSTATIC PRECIPITATOR ; MERCURY EMISSIONS ; FLY-ASH ; COMBUSTION ; BEHAVIOR ; SPECIATION |
资助项目 | Beijing Natural Science Foundation[8192014] ; National Key Research and Development Program of China[2016YFC0208103] |
WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:001177560800001 |
出版者 | ELSEVIER |
资助机构 | Beijing Natural Science Foundation ; National Key Research and Development Program of China |
源URL | [http://ir.igsnrr.ac.cn/handle/311030/203980] ![]() |
专题 | 中国科学院地理科学与资源研究所 |
通讯作者 | Yue, Tao |
作者单位 | 1.Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China 2.Chinese Res Inst Environm Sci, Res Ctr Environm Pollut Control Engn Technol, Beijing 100012, Peoples R China 3.Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China 4.Chinese Acad Sci, Inst Geog Sci & Nat Resources Res, Beijing 100101, Peoples R China 5.Univ Sci & Technol Beijing, 30 Xueyuan Rd, Beijing 100083, Peoples R China |
推荐引用方式 GB/T 7714 | Tong, Yali,Gao, Jiajia,Yue, Tao,et al. Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers[J]. JOURNAL OF HAZARDOUS MATERIALS,2024,466:13. |
APA | Tong, Yali,Gao, Jiajia,Yue, Tao,Yuan, Yue,Tang, Yu,&Wang, Lingqing.(2024).Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers.JOURNAL OF HAZARDOUS MATERIALS,466,13. |
MLA | Tong, Yali,et al."Tracking the flows of Hg, As, Cd, Cr, and Pb in Chinese coal-fired industrial boilers".JOURNAL OF HAZARDOUS MATERIALS 466(2024):13. |
入库方式: OAI收割
来源:地理科学与资源研究所
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