Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose
文献类型：期刊论文
| 作者 | Li, JiaHao; Hou, YuanZhen; He, ZeZhou; Wu HA(吴恒安); Zhu, YinBo |
| 刊名 | NANO LETTERS
 |
| 出版日期 | 2024-05-14 |
| 卷号 | 24期号:21页码:6262-6268 |
| 关键词 | nanocellulose cellulose nanochannel ion transport strain engineering ion cross-linking |
| ISSN号 | 1530-6984 |
| DOI | 10.1021/acs.nanolett.4c00867 |
| 通讯作者 | Zhu, YinBo(zhuyinbo@ustc.edu.cn) |
| 英文摘要 | Expanding the interlayer spacing plays a significant role in improving the conductivity of a cellulose-based conductor. However, it remains a challenge to regulate the cellulose nanochannel expanded by ion coordination. Herein, starting from multiscale mechanics, we proposed a strain engineering method to regulate the interlayer spacing of the cellulose nanochannels. First-principles calculations were conducted to select the most suitable ions for coordination. Large-scale molecular dynamics simulations were performed to reveal the mechanism of interlayer spacing expansion by the ion cross-linking. Combining the shear-lag model, we established the relationship between interfacial cross-link density and interlayer spacing of an ion-coordinated cellulose nanochannel. Consequently, fast ion transport and current regulation were realized via the strain engineering of nanochannels, which provides a promising strategy for the current regulation of a cellulose-based conductor. |
| 分类号 | 一类 |
| WOS关键词 | LENGTH SCALES ; CROSS-LINKING ; GRAPHENE ; LOCALIZATION ; COMPOSITES ; BATTERIES |
| 资助项目 | National Natural Science Foundation of China[2022465] ; Youth Innovation Promotion Association CAS[12232016] ; Youth Innovation Promotion Association CAS[12172346] ; Youth Innovation Promotion Association CAS[12202431] ; National Natural Science Foundation of China[2208085QA24] ; Natural Science Foundation of Anhui Province ; Supercomputing Center of University of Science and Technology of China |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:001225234300001 |
| 资助机构 | National Natural Science Foundation of China ; Youth Innovation Promotion Association CAS ; National Natural Science Foundation of China ; Natural Science Foundation of Anhui Province ; Supercomputing Center of University of Science and Technology of China |
| 其他责任者 | Zhu, YinBo |
| 源URL | [http://dspace.imech.ac.cn/handle/311007/95363]  |
| 专题 | 力学研究所_非线性力学国家重点实验室 |
| 推荐引用方式 GB/T 7714 | Li, JiaHao,Hou, YuanZhen,He, ZeZhou,et al. Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose[J]. NANO LETTERS,2024,24(21):6262-6268. |
| APA | Li, JiaHao,Hou, YuanZhen,He, ZeZhou,吴恒安,&Zhu, YinBo.(2024).Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose.NANO LETTERS,24(21),6262-6268. |
| MLA | Li, JiaHao,et al."Strain Engineering of Ion-Coordinated Nanochannels in Nanocellulose".NANO LETTERS 24.21(2024):6262-6268. |
入库方式： OAI收割
来源：力学研究所
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