Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer
文献类型:期刊论文
| 作者 | Q. Li; X. Xie; H. Wu; H. Chen; W. Wang; X. Kong and Y. Chang |
| 刊名 | Nano Letters
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| 出版日期 | 2023 |
| 卷号 | 23期号:8页码:3444-3450 |
| ISSN号 | 15306984 |
| DOI | 10.1021/acs.nanolett.3c00495 |
| 英文摘要 | Highly doped lanthanide luminescent nanoparticles exhibit unique optical properties, providing exciting opportunities for many ground-breaking applications, such as super-resolution microscopy, deep-tissue bioimaging, confidentiality, and anticounterfeiting. However, the concentration-quenching effect compromises their luminescence efficiency/brightness, hindering their wide range of applications. Herein, we developed a low-temperature suppression cross-relaxation strategy, which drastically enhanced upconversion luminescence (up to 2150-fold of green emission) in Er3+-rich nanosystems. The cryogenic field opens the energy transport channel of Er3+ multiphoton upconversion by further suppressing phonon-assisted cross-relaxation. Our results provide direct evidence for understanding the energy loss mechanism of photon upconversion, deepening a fundamental understanding of the upconversion process in highly doped nanosystems. Furthermore, it also suggests the potential applications of upconversion nanoparticles for extreme ambient-temperature detection and anticounterfeiting. © 2023 American Chemical Society. |
| URL标识 | 查看原文 |
| 源URL | [http://ir.ciomp.ac.cn/handle/181722/67635] ![]() |
| 专题 | 中国科学院长春光学精密机械与物理研究所 |
| 推荐引用方式 GB/T 7714 | Q. Li,X. Xie,H. Wu,et al. Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer[J]. Nano Letters,2023,23(8):3444-3450. |
| APA | Q. Li,X. Xie,H. Wu,H. Chen,W. Wang,&X. Kong and Y. Chang.(2023).Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer.Nano Letters,23(8),3444-3450. |
| MLA | Q. Li,et al."Superenhancement Photon Upconversion Nanoparticles for Photoactivated Nanocryometer".Nano Letters 23.8(2023):3444-3450. |
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