Unconventional correlated insulator in CrOCl-interfaced Bernal bilayer graphene
文献类型:期刊论文
作者 | Yang, Kaining6,7; Gao, Xiang6,7; Wang, Yaning8,9; Zhang, Tongyao6,7; Gao, Yuchen1,2,18; Lu, Xin10; Zhang, Shihao10; Liu, Jianpeng10,14; Gu, Pingfan1,2,18; Luo, Zhaoping8 |
刊名 | NATURE COMMUNICATIONS
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出版日期 | 2023-04-14 |
卷号 | 14期号:1页码:10 |
DOI | 10.1038/s41467-023-37769-2 |
通讯作者 | Lu, Xin(lvxin@shanghaitech.edu.cn) ; Dai, Xi(daix@ust.hk) ; Chen, Jian-Hao(chenjianhao@pku.edu.cn) ; Ye, Yu(ye_yu@pku.edu.cn) ; Han, Zheng(vitto.han@gmail.com) |
英文摘要 | Here, the authors report evidence of unconventional correlated insulating states in bilayer graphene/CrOCl heterostructures over wide doping ranges and demonstrate their application for the realization of low-temperature logic inverters. The realization of graphene gapped states with large on/off ratios over wide doping ranges remains challenging. Here, we investigate heterostructures based on Bernal-stacked bilayer graphene (BLG) atop few-layered CrOCl, exhibiting an over-1-G omega-resistance insulating state in a widely accessible gate voltage range. The insulating state could be switched into a metallic state with an on/off ratio up to 10(7) by applying an in-plane electric field, heating, or gating. We tentatively associate the observed behavior to the formation of a surface state in CrOCl under vertical electric fields, promoting electron-electron (e-e) interactions in BLG via long-range Coulomb coupling. Consequently, at the charge neutrality point, a crossover from single particle insulating behavior to an unconventional correlated insulator is enabled, below an onset temperature. We demonstrate the application of the insulating state for the realization of a logic inverter operating at low temperatures. Our findings pave the way for future engineering of quantum electronic states based on interfacial charge coupling. |
资助项目 | National Key R&D Program of China[2019YFA0307800] ; National Key R&D Program of China[2017YFA0206301] ; National Key R&D Program of China[2018YFA0306900] ; National Key R&D Program of China[2019YFA0308402] ; National Key R&D Program of China[2018YFA0305604] ; National Natural Science Foundation of China (NSFC)[92265203] ; National Natural Science Foundation of China (NSFC)[11974357] ; National Natural Science Foundation of China (NSFC)[U1932151] ; National Natural Science Foundation of China (NSFC)[11934001] ; National Natural Science Foundation of China (NSFC)[11774010] ; National Natural Science Foundation of China (NSFC)[92265106] ; National Natural Science Foundation of China (NSFC)[11921005] ; Elemental Strategy Initiative ; MEXT, Japan[JPMXP0112101001] ; JSPS KAKENHI[JP20H00354] ; A3 Foresight by JSPS ; Beijing Municipal Natural Science Foundation[JQ20002] |
WOS研究方向 | Science & Technology - Other Topics |
语种 | 英语 |
WOS记录号 | WOS:000969250300021 |
出版者 | NATURE PORTFOLIO |
资助机构 | National Key R&D Program of China ; National Natural Science Foundation of China (NSFC) ; Elemental Strategy Initiative ; MEXT, Japan ; JSPS KAKENHI ; A3 Foresight by JSPS ; Beijing Municipal Natural Science Foundation |
源URL | [http://ir.imr.ac.cn/handle/321006/177695] ![]() |
专题 | 金属研究所_中国科学院金属研究所 |
通讯作者 | Lu, Xin; Dai, Xi; Chen, Jian-Hao; Ye, Yu; Han, Zheng |
作者单位 | 1.Peking Univ, Sch Phys, State Key Lab Mesoscop Phys, Beijing, Peoples R China 2.Peking Univ, Sch Phys, Frontiers Sci Ctr Nano Optoelect, Beijing, Peoples R China 3.Hefei Natl Lab, Hefei, Peoples R China 4.Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Japan 5.Peking Univ, Key Lab Phys & Chem Nanodevices, Beijing, Peoples R China 6.Shanxi Univ, Inst Optoelect, State Key Lab Quantum Opt & Quantum Opt Devices, Taiyuan, Peoples R China 7.Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan, Peoples R China 8.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang, Peoples R China 9.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei, Anhui, Peoples R China 10.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai, Peoples R China |
推荐引用方式 GB/T 7714 | Yang, Kaining,Gao, Xiang,Wang, Yaning,et al. Unconventional correlated insulator in CrOCl-interfaced Bernal bilayer graphene[J]. NATURE COMMUNICATIONS,2023,14(1):10. |
APA | Yang, Kaining.,Gao, Xiang.,Wang, Yaning.,Zhang, Tongyao.,Gao, Yuchen.,...&Han, Zheng.(2023).Unconventional correlated insulator in CrOCl-interfaced Bernal bilayer graphene.NATURE COMMUNICATIONS,14(1),10. |
MLA | Yang, Kaining,et al."Unconventional correlated insulator in CrOCl-interfaced Bernal bilayer graphene".NATURE COMMUNICATIONS 14.1(2023):10. |
入库方式: OAI收割
来源:金属研究所
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