Experimental Research System and Efficiency Evaluation Method of CO2 Sequestration in Basalt Mineralization
文献类型：期刊论文
| 作者 | Wang, Yaping4; Chen, Ying3,4; Wang, Wenyang3; Jiang, Fujie4; Dou WC(窦文超)2; Su, Min1; Bao, Zhidong4 |
| 刊名 | ENERGY & FUELS
 |
| 出版日期 | 2024-07-22 |
| 卷号 | 38期号:15页码:14414-14421 |
| ISSN号 | 0887-0624 |
| DOI | 10.1021/acs.energyfuels.4c00677 |
| 通讯作者 | Chen, Ying(2021215016@student.cup.edu.cn) ; Wang, Wenyang(wywang@mail.iggcas.ac.cn) |
| 英文摘要 | Basalt offers a promising method for safe and permanent CO2 storage on a large scale. Currently, most experiments focus on the reactivity and mineralization kinetics of basalt and CO2, often without accurately quantifying the reactions or considering the influence of carbonate rocks present in basalt, leading to inaccurate and complex results. The study conducted CO2 water-rock reaction experiments under various conditions using a self-designed high-temperature and high-pressure reactor. The qualitative verification of changes before and after the reaction was done using X-ray diffraction (XRD) and scanning electron microscopy with an energy-dispersive spectrometer (SEM-EDS). Subsequently, the mineralization reaction efficiency was calculated by refining pressure data and a numerical model, and the results were validated using the improved total inorganic carbon (TIC) method. The results indicated the following: (1) various forms of calcium carbonate crystals were observed and confirmed post mineralization reaction. (2) Following the reaction, the feldspar and pyroxene in basalt decreased, the calcite content slightly increased, and a new amorphous phase formed. (3) Mineralization efficiency was assessed by combining pressure data from the instrument with a numerical model. The calculation results of the carbon sequestration efficiency (CSE) were consistent with the TIC method, confirming the system's reliability. This method effectively addresses the issues of inaccurate and complex mineralization reaction efficiency evaluation and can contribute to research on basalt-CO2 reaction ability and mineralization reaction kinetics. |
| 分类号 | 二类/Q1 |
| WOS关键词 | CARBON-DIOXIDE ; STORAGE ; DISSOLUTION ; KINETICS ; ROCKS ; DISPOSAL |
| 资助项目 | Autonomous Deployment of Scientific Research Projects by the Institute of Geology and Geophysics, Chinese Academy of Sciences[IGGCAS-202201] ; Open Fund Project of the State Key Laboratory of Lithospheric Evolution[SKL-Z202103] |
| WOS研究方向 | Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001274524400001 |
| 资助机构 | Autonomous Deployment of Scientific Research Projects by the Institute of Geology and Geophysics, Chinese Academy of Sciences ; Open Fund Project of the State Key Laboratory of Lithospheric Evolution |
| 其他责任者 | Chen, Ying ; Wang, Wenyang |
| 源URL | [http://dspace.imech.ac.cn/handle/311007/96157]  |
| 专题 | 力学研究所_流固耦合系统力学重点实验室(2012-) |
| 作者单位 | 1.China Univ Petr, Coll Geophys, Beijing 102249, Peoples R China 2.Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China; 3.Chinese Acad Sci, Inst Geol & Geophys, Key Lab Petr Resource Res, Beijing 100029, Peoples R China; 4.China Univ Petr, Coll Geosci, Beijing 102249, Peoples R China; |
| 推荐引用方式 GB/T 7714 | Wang, Yaping,Chen, Ying,Wang, Wenyang,et al. Experimental Research System and Efficiency Evaluation Method of CO2 Sequestration in Basalt Mineralization[J]. ENERGY & FUELS,2024,38(15):14414-14421. |
| APA | Wang, Yaping.,Chen, Ying.,Wang, Wenyang.,Jiang, Fujie.,窦文超.,...&Bao, Zhidong.(2024).Experimental Research System and Efficiency Evaluation Method of CO2 Sequestration in Basalt Mineralization.ENERGY & FUELS,38(15),14414-14421. |
| MLA | Wang, Yaping,et al."Experimental Research System and Efficiency Evaluation Method of CO2 Sequestration in Basalt Mineralization".ENERGY & FUELS 38.15(2024):14414-14421. |
入库方式： OAI收割
来源：力学研究所
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