Impacts of dust events on chemical characterization and associated source contributions of atmospheric particulate matter in northern China
文献类型：期刊论文
| 作者 | Li, Ruiyu1,2; Zhang, Miao3; Du, Yuming4; Wang, Guixia3; Shang, Chunlin4; Liu, Yao4; Zhang, Min4; Meng, Qingpeng2; Cui, Min5; Yan, Caiqing1,2 |
| 刊名 | ENVIRONMENTAL POLLUTION
 |
| 出版日期 | 2023 |
| 卷号 | 316页码:12 |
| 关键词 | Dust event Particulate matter Chemical composition Sources PMF model Crustal materials |
| ISSN号 | 0269-7491 |
| DOI | 10.1016/j.envpol.2022.120597 |
| 英文摘要 | Sand and dust have significant impacts on air quality, climate, and human health. To investigate the influences of dust storms on chemical characterization and source contributions of fine particulate matter (PM2.5) in areas with different distances from dust source regions, PM2.5 and associated chemical composition were measured in two industrial cities with one near sand sources (i.e., Wuhai) and the other far from sand sources (i.e., Jinan) in northern China in March 2021. Results showed that PM mass concentrations significantly increased and exceeded the Chinese National Ambient Air Quality standard during the dust events, with absolute concentrations and fractional contributions of PM2.5-bound crustal and trace elements increased while secondary inorganic ions decreased at both sites. Crustal materials dominated the increased PM2.5 mass from non-dust period to dust period in both cities. These were further evidenced by PM2.5 source apportionment results from positive matrix factorization model. During the dust events, dust sources contributed up to 88% of PM2.5 mass in Wuhai and -38% of PM2.5 mass in Jinan, a city about thousands of kilometers away from the sand source. Besides, the measurement data indicated that dust from northwest China may also bring along with high abundance of organic matter and vanadium. Secondary and traffic sources were two of the most important source contributors to PM2.5 in both cities during the non-dust periods. However, the near sand source city was more susceptible to the aggravating effects of dust and minerals, with much higher contributions by crustal materials (-47%, from the aspect of chemical components) and dust-related sources (-26%, from the aspect of sources) to PM2.5 mass even during non-dust periods. This study highlighted the urgent need for more action and effective control of sand sources to reduce the impact on air quality in downstream regions. |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000904789500006 |
| 源URL | [http://ir.gig.ac.cn/handle/344008/71506]  |
| 专题 | 中国科学院广州地球化学研究所 |
| 通讯作者 | Yan, Caiqing |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Prov Key Lab Environm Protect & Resource, Guangzhou 510640, Peoples R China 2.Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China 3.Shandong Prov Ecoenvironm Monitoring Ctr, Jinan 250101, Peoples R China 4.Inner Mongolia Autonomous Reg Environm Monitoring, Wuhai Branch, Wuhai 016000, Peoples R China 5.Yangzhou Univ, Coll Environm Sci & Engn, Yangzhou 225009, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Ruiyu,Zhang, Miao,Du, Yuming,et al. Impacts of dust events on chemical characterization and associated source contributions of atmospheric particulate matter in northern China[J]. ENVIRONMENTAL POLLUTION,2023,316:12. |
| APA | Li, Ruiyu.,Zhang, Miao.,Du, Yuming.,Wang, Guixia.,Shang, Chunlin.,...&Yan, Caiqing.(2023).Impacts of dust events on chemical characterization and associated source contributions of atmospheric particulate matter in northern China.ENVIRONMENTAL POLLUTION,316,12. |
| MLA | Li, Ruiyu,et al."Impacts of dust events on chemical characterization and associated source contributions of atmospheric particulate matter in northern China".ENVIRONMENTAL POLLUTION 316(2023):12. |
入库方式： OAI收割
来源：广州地球化学研究所
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