Occurrence and carcinogenic potential of airborne PBDD/Fs and PCDD/Fs around a large-scale municipal solid waste incinerator: A long-term passive air sampling study
文献类型：期刊论文
| 作者 | Li, Hui-Ru3,4,5,6,8; Liu, Ming-Yang5,6,7; Hu, Jun-Jie2; Song, Ai-Min5,6,7; Peng, Ping-An1,5,6,7,9; Ying, Guang Guo3,4; Yan, Bo3,4; Chen, Tao3,4 |
| 刊名 | ENVIRONMENT INTERNATIONAL
 |
| 出版日期 | 2023-08-01 |
| 卷号 | 178页码:12 |
| 关键词 | Persistent organic pollutants Dioxins and furans Positive matrix factorization Toxic equivalent quantity (TEQ) Aryl hydrocarbon receptor (AhR) |
| ISSN号 | 0160-4120 |
| DOI | 10.1016/j.envint.2023.108104 |
| 英文摘要 | Municipal solid waste incinerator (MSWI) not only is deemed one of the uppermost sources of polychlorinated dibenzo-p-dioxins/furans (PCDD/Fs), but also produces substantial amount of polybrominated dibenzo-p-dioxins/furans (PBDD/Fs) owing to the existence of brominated flame retardants (BFRs) in the waste. So far, however, PBDD/Fs in the vicinal environments of MSWI and their associated risks remain rarely studied. Based on a one-year passive air sampling (PAS) scheme, we investigated airborne PBDD/Fs and PCDD/Fs around a large-scale MSWI that has been operated for multi-years. Both the concentrations of PBDD/Fs and PCDD/Fs showed spatially decreasing trends with the distance away from the MSWI, confirming the influence of the MSWI on the dioxin levels in its ambient air. But its influence on PBDD/Fs was less because PBDD/Fs exhibit lower volatility and therefore lower gaseous concentrations than PCDD/Fs. Compared to the existing global data of airborne PCDD/Fs and PBDD/Fs, our data of the MSWI vicinity were at medium levels, despite PAS samples only represent the concentrations of gaseous dioxins in theory. The seasonal data suggest that meteorological conditions exerted apparent influences over the concentrations and sources of airborne dioxins around the MSWI. As for PCDD/Fs, the MSWI was diagnosed as their uppermost source, followed by local traffic and volatilization/deposition. Whereas the top three PBDD/F sources were related to PBDEs, bromophenol/bromobenzene, and traffic vehicles, respectively. The bioassay-derived TEQs based on the aryl hydrocarbon receptor activation of airborne dioxins around the MSWI were one or two orders of magnitudes higher than their concentration-based TEQs, and the corresponding carcinogenic risks at some MSWI-vicinal sites exceeded the acceptable threshold proposed by the U. S. EPA (10(-6) similar to 10(-4)) and deserve continuous attention. |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001048483700001 |
| 源URL | [http://ir.gig.ac.cn/handle/344008/74655]  |
| 专题 | 有机地球化学国家重点实验室 |
| 通讯作者 | Li, Hui-Ru |
| 作者单位 | 1.Guangdong Hong Kong Macao Joint Lab Environm Pollu, Guangzhou 510640, Peoples R China 2.Dongguan Univ Technol, Sch Environm & Civil Engn, Dongguan 523808, Peoples R China 3.South China Normal Univ, SCNU Environm Res Inst, Sch Environm, Guangdong Prov Key Lab Chem Pollut & Environm Safe, Guangzhou 510006, Peoples R China 4.South China Normal Univ, Sch Environm, MOE Key Lab Theoret Chem Environm, Guangzhou 510006, Peoples R China 5.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China 6.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Key Lab Environm Protect & Resources Uti, Guangzhou 510640, Peoples R China 7.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 8.Sci Bldg 3,378 Waihuan West Rd, Guangzhou 510006, Peoples R China 9.CAS Ctr Excellence Deep Earth Sci, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Hui-Ru,Liu, Ming-Yang,Hu, Jun-Jie,et al. Occurrence and carcinogenic potential of airborne PBDD/Fs and PCDD/Fs around a large-scale municipal solid waste incinerator: A long-term passive air sampling study[J]. ENVIRONMENT INTERNATIONAL,2023,178:12. |
| APA | Li, Hui-Ru.,Liu, Ming-Yang.,Hu, Jun-Jie.,Song, Ai-Min.,Peng, Ping-An.,...&Chen, Tao.(2023).Occurrence and carcinogenic potential of airborne PBDD/Fs and PCDD/Fs around a large-scale municipal solid waste incinerator: A long-term passive air sampling study.ENVIRONMENT INTERNATIONAL,178,12. |
| MLA | Li, Hui-Ru,et al."Occurrence and carcinogenic potential of airborne PBDD/Fs and PCDD/Fs around a large-scale municipal solid waste incinerator: A long-term passive air sampling study".ENVIRONMENT INTERNATIONAL 178(2023):12. |
入库方式： OAI收割
来源：广州地球化学研究所
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