Organophosphate esters (OPEs) in a heavily polluted river in South China: Occurrence, spatiotemporal trends, sources, and phase distribution
文献类型：期刊论文
| 作者 | Liu, Yi-Shan4,6; Li, Hui-Ru4,6,7; Lao, Zhi-Lang4,6; Ma, Sheng-Tao5; Liao, Zi-Cong4,6; Song, Ai-Min1,2,3; Liu, Ming-Yang1,2,3; Liu, You-Sheng4,6; Ying, Guang-Guo4,6 |
| 刊名 | ENVIRONMENTAL POLLUTION
 |
| 出版日期 | 2023-11-01 |
| 卷号 | 336页码:12 |
| 关键词 | Organophosphorus flame retardant Emerging contaminants Plasticizer Positive matrix factorization (PMF) E-waste recycling Temporal trend |
| ISSN号 | 0269-7491 |
| DOI | 10.1016/j.envpol.2023.122492 |
| 英文摘要 | In the past decade, organophosphate esters (OPEs) undergo rapid increase in production and use. Meanwhile, owing to their additive property, OPEs exhibit liability to escape from related products and therefore ubiquity in various environments. Moreover, numerous researches verify their bioavailability and negative effects on biota and human, hence their occurrence and associated risks have caught much concern, particularly those in aquatic systems. So far, however, OPEs in water are generally investigated as a whole, their phase distribution and behavior in waterbodies are incompletely characterized. We examined 25 OPEs in water (including dissolved and particulate phases), sediment, and sediment core samples from the Lian River, which flows through the Guiyu ewaste recycling zone and Shantou specific economic zone in South China. Compared to most global waterbodies, the Lian River showed high or ultrahigh OPE levels in both water and sediments, particularly in the reaches surrounded by e-waste recycling and plastic-related industries, which were the top two greatest OPE sources. Non-industrial and agriculture-related anthropogenic activities also contributed OPEs. Sediment core data suggested that OPEs have been present in waters in Guiyu since the 1960s and showed a temporal trend consistent with the local waste-recycling business. The phase distribution of OPEs in the Lian River was significantly correlated with their hydrophobicity and solubility. Owing to their wide range of physicochemical properties, OPE congeners showed significant percentage differences in the Lian River water and sediments. Generally, OPEs in water reflect their dynamic real-time inputs, while those in sediment signify their accumulative deposition, which is another cause of their phase distribution disparities in the Lian River. The physicochemical parameters of OPEs first imposed negative and then positive influences on their dissolved phase-sediment distribution, indicating the involvement of both the adsorption of dissolved OPEs and the deposition of particle-bound OPEs. |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001070340300001 |
| 源URL | [http://ir.gig.ac.cn/handle/344008/74846]  |
| 专题 | 有机地球化学国家重点实验室 |
| 通讯作者 | Li, Hui-Ru |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Key Lab Environm Protect & Resources Uti, Guangzhou 510640, Peoples R China 3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 4.South China Normal Univ, Sch Environm, MOE Key Lab Theoret Chem Environm, Guangzhou 510006, Peoples R China 5.Guangzhou Med Univ, Sch Publ Hlth, Guangzhou 511436, Peoples R China 6.South China Normal Univ, SCNU Environm Res Inst, Sch Environm, Guangdong Prov Key Lab Chem Pollut & Environm Safe, Guangzhou 510006, Peoples R China 7.Guangzhou Univ Town, Sci Bldg 3,378 Waihuan West Rd, Guangzhou 510006, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Yi-Shan,Li, Hui-Ru,Lao, Zhi-Lang,et al. Organophosphate esters (OPEs) in a heavily polluted river in South China: Occurrence, spatiotemporal trends, sources, and phase distribution[J]. ENVIRONMENTAL POLLUTION,2023,336:12. |
| APA | Liu, Yi-Shan.,Li, Hui-Ru.,Lao, Zhi-Lang.,Ma, Sheng-Tao.,Liao, Zi-Cong.,...&Ying, Guang-Guo.(2023).Organophosphate esters (OPEs) in a heavily polluted river in South China: Occurrence, spatiotemporal trends, sources, and phase distribution.ENVIRONMENTAL POLLUTION,336,12. |
| MLA | Liu, Yi-Shan,et al."Organophosphate esters (OPEs) in a heavily polluted river in South China: Occurrence, spatiotemporal trends, sources, and phase distribution".ENVIRONMENTAL POLLUTION 336(2023):12. |
入库方式： OAI收割
来源：广州地球化学研究所
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