中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Char dominates black carbon aerosol emission and its historic reduction in China

文献类型:期刊论文

作者Cai, Junjie2; Jiang, Hongxing2; Chen, Yingjun2,3; Liu, Zeyu2; Han, Yong2; Shen, Huizhong4; Song, Jianzhong5,6; Li, Jun5,6; Zhang, Yanlin1,7; Wang, Rong2
刊名NATURE COMMUNICATIONS
出版日期2023-10-13
卷号14期号:1页码:9
DOI10.1038/s41467-023-42192-8
英文摘要Emission factors and inventories of black carbon (BC) aerosols are crucial for estimating their adverse atmospheric effect. However, it is imperative to separate BC emissions into char and soot subgroups due to their significantly different physicochemical properties and potential effects. Here, we present a substantial dataset of char and soot emission factors derived from field and laboratory measurements. Based on the latest results of the char-to-soot ratio, we further reconstructed the emission inventories of char and soot for the years 1960-2017 in China. Our findings indicate that char dominates annual BC emissions and its huge historical reduction, which can be attributable to the rapid changes in energy structure, combustion technology and emission standards in recent decades. Our results suggest that further BC emission reductions in both China and the world should focus on char, which mainly derives from lower-temperature combustion and is easier to decrease compared to soot.
WOS研究方向Science & Technology - Other Topics
语种英语
WOS记录号WOS:001117712600035
源URL[http://ir.gig.ac.cn/handle/344008/76258]  
专题有机地球化学国家重点实验室
通讯作者Chen, Yingjun; Zhang, Gan
作者单位1.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Int Joint Lab Climate & Environm Change ILCEC, Nanjing 210044, Peoples R China
2.Fudan Univ, Shanghai Key Lab Atmospher Particle Pollut & Prev, Dept Environm Sci & Engn, Shanghai 200438, Peoples R China
3.Shanghai Inst Pollut Control & Ecol Secur, Shanghai 200092, Peoples R China
4.Southern Univ Sci & Technol, Sch Environm Sci & Engn, Guangdong Prov Observat & Res Stn Coastal Atmosph, Shenzhen 518055, Peoples R China
5.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China
6.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Hong Kong Macao Joint Lab Environm Poll, Guangzhou 510640, Peoples R China
7.Nanjing Univ Informat Sci & Technol, Coll Appl Meteorol, Jiangsu Prov Key Lab Agr Meteorol, Nanjing 210044, Peoples R China
推荐引用方式
GB/T 7714
Cai, Junjie,Jiang, Hongxing,Chen, Yingjun,et al. Char dominates black carbon aerosol emission and its historic reduction in China[J]. NATURE COMMUNICATIONS,2023,14(1):9.
APA Cai, Junjie.,Jiang, Hongxing.,Chen, Yingjun.,Liu, Zeyu.,Han, Yong.,...&Zhang, Gan.(2023).Char dominates black carbon aerosol emission and its historic reduction in China.NATURE COMMUNICATIONS,14(1),9.
MLA Cai, Junjie,et al."Char dominates black carbon aerosol emission and its historic reduction in China".NATURE COMMUNICATIONS 14.1(2023):9.

入库方式: OAI收割

来源:广州地球化学研究所

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