Measurement report: Atmospheric ice nuclei in the Changbai Mountains (2623 m a.s.l.) in northeastern Asia
文献类型：期刊论文
| 作者 | Sun, Yue2; Zhu, Yujiao2; Qi, Yanbin1; Chen, Lanxiadi4; Mu, Jiangshan2; Shan, Ye2; Yang, Yu2; Nie, Yanqiu2; Liu, Ping2; Cui, Can2 |
| 刊名 | ATMOSPHERIC CHEMISTRY AND PHYSICS
 |
| 出版日期 | 2024-03-15 |
| 卷号 | 24期号:5页码:3241-3256 |
| ISSN号 | 1680-7316 |
| DOI | 10.5194/acp-24-3241-2024 |
| 英文摘要 | Atmospheric ice nucleation plays an important role in modulating the global hydrological cycle and atmospheric radiation balance. To date, few comprehensive field observations of ice nuclei have been carried out at high-altitude sites, which are close to the height of mixed-phase cloud formation. In this study, we measured the concentration of ice-nucleating particles (INPs) in the immersion freezing mode at the summit of the Changbai Mountains (2623 m above sea level), northeast Asia, in summer 2021. The cumulative number concentration of INPs varied from 1.6 x 10(-3) to 78.3 L-1 over the temperature range of -5.5 to -29.0 degrees C. Proteinaceous-based biological materials accounted for the majority of INPs, with the proportion of biological INPs (bio-INPs) exceeding 67 % across the entire freezing-temperature range, with this proportion even exceeding 90 % above -13.0 degrees C. At freezing temperatures ranging from -11.0 to -8.0 degrees C, bio-INPs were found to significantly correlate with wind speed (r = 0.5-0.8, p < 0.05) and Ca2+ (r = 0.6-0.9), and good but not significant correlation was found with isoprene (r = 0.6-0.7) and its oxidation products (isoprene x O-3) (r = 0.7), suggesting that biological aerosols may attach to or mix with soil dust and contribute to INPs. During the daytime, bio-INPs showed a positive correlation with the planetary boundary layer (PBL) height at freezing temperatures ranging from -22.0 to -19.5 degrees C (r > 0.7, p < 0.05), with the valley breezes from southern mountainous regions also influencing the concentration of INPs. Moreover, the long-distance transport of air mass from the Japan Sea and South Korea significantly contributed to the high concentrations of bio-INPs. Our study emphasizes the important role of biological sources of INPs in the high-altitude atmosphere of northeastern Asia and the significant contribution of long-range transport to the INP concentrations in this region. |
| WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| WOS记录号 | WOS:001190654800001 |
| 源URL | [http://ir.gig.ac.cn/handle/344008/77166]  |
| 专题 | 有机地球化学国家重点实验室 |
| 通讯作者 | Zhu, Yujiao; Xue, Likun |
| 作者单位 | 1.Jilin Prov Technol Ctr Meteorol Disaster Prevent, Changchun 130062, Peoples R China 2.Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China 3.Changbai Mt Meteorol Observ, Jilin 133613, Peoples R China 4.Guangzhou Inst Geochem, Chinese Acad Sci, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Sun, Yue,Zhu, Yujiao,Qi, Yanbin,et al. Measurement report: Atmospheric ice nuclei in the Changbai Mountains (2623 m a.s.l.) in northeastern Asia[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2024,24(5):3241-3256. |
| APA | Sun, Yue.,Zhu, Yujiao.,Qi, Yanbin.,Chen, Lanxiadi.,Mu, Jiangshan.,...&Xue, Likun.(2024).Measurement report: Atmospheric ice nuclei in the Changbai Mountains (2623 m a.s.l.) in northeastern Asia.ATMOSPHERIC CHEMISTRY AND PHYSICS,24(5),3241-3256. |
| MLA | Sun, Yue,et al."Measurement report: Atmospheric ice nuclei in the Changbai Mountains (2623 m a.s.l.) in northeastern Asia".ATMOSPHERIC CHEMISTRY AND PHYSICS 24.5(2024):3241-3256. |
入库方式： OAI收割
来源：广州地球化学研究所
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