Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs
文献类型:期刊论文
作者 | Yu, Huimin2,3,6; Lin, Tian4; Hu, Limin5; Lammel, Gerhard6,7; Zhao, Shizhen1,8; Sun, Xueshi2; Wu, Xiao5; Guo, Zhigang2,3 |
刊名 | ENVIRONMENTAL POLLUTION
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出版日期 | 2023-12-01 |
卷号 | 338页码:10 |
关键词 | Polychlorinated biphenyls Long-range atmospheric transport Riverine input East China marginal seas Unintentionally-produced PCBs |
ISSN号 | 0269-7491 |
DOI | 10.1016/j.envpol.2023.122707 |
英文摘要 | The production and use of intentionally-produced polychlorinated biphenyls (PCBs) in China have a short history compared with countries of North America and Europe, where technical PCB mixtures were manufactured in large amounts for decades before being banned. Unintentionally-produced PCB emissions increased dramatically in China, leading to unique profiles of PCB burdens. This study first time evaluated 208 individual PCB congeners at 94 sites from surface sediments of the East China Marginal Seas (ECMSs) and explored their sources. Non-technical PCBs transported from atmospheric transport and river discharge played a dominant role in most areas of the ECMSs, while historical residuals of technical PCBs occupied the fine-grained sediments in muddy areas of the central Yellow Sea (YS), regarding to the low sedimentation rate in the central YS. Furthermore, emissions from Taizhou located on the coast of the East China Sea (ECS), which is an important electronic waste dismantling site in East China, contributed additional technical PCBs to the inner shelf of the ECS. Our results indicate that non-technical PCBs have become the dominant PCB species in the ECMSs, and emphasize the synergistic effects of large riverine input, long-range atmospheric transport, and muddy shelf deposition on PCB source and sink of in marginal seas. |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:001096055400001 |
源URL | [http://ir.gig.ac.cn/handle/344008/78895] ![]() |
专题 | 有机地球化学国家重点实验室 |
通讯作者 | Guo, Zhigang |
作者单位 | 1.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Prov Key Lab Environm Protect & Resource, Guangdong Hong Kong Macao Joint Lab Environm Pollu, Guangzhou 510640, Peoples R China 2.Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Preve, Natl Observat & Res Stn Wetland Ecosyst Yangtze Es, Shanghai 200433, Peoples R China 3.Inst Ecochongming IEC, Shanghai 202162, Peoples R China 4.Shanghai Ocean Univ, Coll Marine Ecol & Environm, Shanghai 201306, Peoples R China 5.Ocean Univ China, Key Lab Submarine Geosci & Technol, MOE, Qingdao 266100, Peoples R China 6.Max Planck Inst Chem, Multiphase Chem Dept, D-55128 Mainz, Germany 7.Masaryk Univ, Fac Sci, RECETOX, Brno 62500, Czech Republic 8.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China |
推荐引用方式 GB/T 7714 | Yu, Huimin,Lin, Tian,Hu, Limin,et al. Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs[J]. ENVIRONMENTAL POLLUTION,2023,338:10. |
APA | Yu, Huimin.,Lin, Tian.,Hu, Limin.,Lammel, Gerhard.,Zhao, Shizhen.,...&Guo, Zhigang.(2023).Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs.ENVIRONMENTAL POLLUTION,338,10. |
MLA | Yu, Huimin,et al."Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs".ENVIRONMENTAL POLLUTION 338(2023):10. |
入库方式: OAI收割
来源:广州地球化学研究所
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