中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs

文献类型:期刊论文

作者Yu, Huimin2,3,6; Lin, Tian4; Hu, Limin5; Lammel, Gerhard6,7; Zhao, Shizhen1,8; Sun, Xueshi2; Wu, Xiao5; Guo, Zhigang2,3
刊名ENVIRONMENTAL POLLUTION
出版日期2023-12-01
卷号338页码:10
关键词Polychlorinated biphenyls Long-range atmospheric transport Riverine input East China marginal seas Unintentionally-produced PCBs
ISSN号0269-7491
DOI10.1016/j.envpol.2023.122707
英文摘要The production and use of intentionally-produced polychlorinated biphenyls (PCBs) in China have a short history compared with countries of North America and Europe, where technical PCB mixtures were manufactured in large amounts for decades before being banned. Unintentionally-produced PCB emissions increased dramatically in China, leading to unique profiles of PCB burdens. This study first time evaluated 208 individual PCB congeners at 94 sites from surface sediments of the East China Marginal Seas (ECMSs) and explored their sources. Non-technical PCBs transported from atmospheric transport and river discharge played a dominant role in most areas of the ECMSs, while historical residuals of technical PCBs occupied the fine-grained sediments in muddy areas of the central Yellow Sea (YS), regarding to the low sedimentation rate in the central YS. Furthermore, emissions from Taizhou located on the coast of the East China Sea (ECS), which is an important electronic waste dismantling site in East China, contributed additional technical PCBs to the inner shelf of the ECS. Our results indicate that non-technical PCBs have become the dominant PCB species in the ECMSs, and emphasize the synergistic effects of large riverine input, long-range atmospheric transport, and muddy shelf deposition on PCB source and sink of in marginal seas.
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:001096055400001
源URL[http://ir.gig.ac.cn/handle/344008/78895]  
专题有机地球化学国家重点实验室
通讯作者Guo, Zhigang
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, Guangdong Prov Key Lab Environm Protect & Resource, Guangdong Hong Kong Macao Joint Lab Environm Pollu, Guangzhou 510640, Peoples R China
2.Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Preve, Natl Observat & Res Stn Wetland Ecosyst Yangtze Es, Shanghai 200433, Peoples R China
3.Inst Ecochongming IEC, Shanghai 202162, Peoples R China
4.Shanghai Ocean Univ, Coll Marine Ecol & Environm, Shanghai 201306, Peoples R China
5.Ocean Univ China, Key Lab Submarine Geosci & Technol, MOE, Qingdao 266100, Peoples R China
6.Max Planck Inst Chem, Multiphase Chem Dept, D-55128 Mainz, Germany
7.Masaryk Univ, Fac Sci, RECETOX, Brno 62500, Czech Republic
8.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China
推荐引用方式
GB/T 7714
Yu, Huimin,Lin, Tian,Hu, Limin,et al. Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs[J]. ENVIRONMENTAL POLLUTION,2023,338:10.
APA Yu, Huimin.,Lin, Tian.,Hu, Limin.,Lammel, Gerhard.,Zhao, Shizhen.,...&Guo, Zhigang.(2023).Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs.ENVIRONMENTAL POLLUTION,338,10.
MLA Yu, Huimin,et al."Sources of polychlorinated biphenyls (PCBs) in sediments of the East China marginal seas: Role of unintentionally-produced PCBs".ENVIRONMENTAL POLLUTION 338(2023):10.

入库方式: OAI收割

来源:广州地球化学研究所

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