中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Multiple Sulfur Isotopes of Iron Sulfides From Thick Greigite-Bearing Sediments Indicate Anaerobic Oxidation and Possible Leakages of Coastal Methane

文献类型:期刊论文

作者Yu, Xiaoxiao2,6; Mei, Xi1; Liu, Jianxing4,5; Lin, Jiarui2,3,6; Wei, Gangjian2,6; Shi, Xuefa4,5; Bai, Jianghao2,3,6; Lin, Mang2,3,6
刊名GEOPHYSICAL RESEARCH LETTERS
出版日期2023-08-28
卷号50期号:16页码:11
关键词greigite pyrite multiple sulfur isotopes coastal methane South Yellow Sea AOM-SR
ISSN号0094-8276
DOI10.1029/2023GL103303
英文摘要Magnetic greigite may be a valuable indicator for methane emissions in the geological past, if its formation pathway and diagenetic environment can be unambiguously defined. Here, we investigate sulfur isotopic compositions of iron sulfides and ferrous iron concentrations of thick greigite-bearing sediments (TGBSs) in the South Yellow Sea, a shallow marginal sea with strong methane emissions. For the first time, isotopically heavy iron sulfides (up to 28.7%0 in delta S-34 and 0.19%0 in Delta S-33) and enrichments of ferrous iron in the TGBSs are observed. We interpret the data as indicating synchronic occurrences of anaerobic oxidation of methane coupled to sulfate and iron reductions, which occur in coastal methanic zones with limited sulfate availability and therefore probably imply leakages of methane. Consequently, we suggest that greigite is a promising geological indicator for tracing methane liberated from coastal sediments, accounting for similar to 60% of the currently rising global marine methane budget.
WOS研究方向Geology
语种英语
WOS记录号WOS:001057745900002
源URL[http://ir.gig.ac.cn/handle/344008/74792]  
专题同位素地球化学国家重点实验室
通讯作者Liu, Jianxing; Lin, Mang
作者单位1.China Geol Survey, Qingdao Inst Marine Geol, Qingdao 266071, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, CAS Ctr Excellence Deep Earth Sci, Guangzhou, Peoples R China
3.Univ Chinese Acad Sci, Beijing, Peoples R China
4.Pilot Natl Lab Marine Sci & Technol, Lab Marine Geol, Qingdao, Peoples R China
5.Minist Nat Resources, Inst Oceanog 1, Key Lab Marine Geol & Metallogeny, Qingdao, Peoples R China
6.Chinese Acad Sci, State Key Lab Isotope Geochem, Guangzhou Inst Geochem, Guangzhou, Peoples R China
推荐引用方式
GB/T 7714
Yu, Xiaoxiao,Mei, Xi,Liu, Jianxing,et al. Multiple Sulfur Isotopes of Iron Sulfides From Thick Greigite-Bearing Sediments Indicate Anaerobic Oxidation and Possible Leakages of Coastal Methane[J]. GEOPHYSICAL RESEARCH LETTERS,2023,50(16):11.
APA Yu, Xiaoxiao.,Mei, Xi.,Liu, Jianxing.,Lin, Jiarui.,Wei, Gangjian.,...&Lin, Mang.(2023).Multiple Sulfur Isotopes of Iron Sulfides From Thick Greigite-Bearing Sediments Indicate Anaerobic Oxidation and Possible Leakages of Coastal Methane.GEOPHYSICAL RESEARCH LETTERS,50(16),11.
MLA Yu, Xiaoxiao,et al."Multiple Sulfur Isotopes of Iron Sulfides From Thick Greigite-Bearing Sediments Indicate Anaerobic Oxidation and Possible Leakages of Coastal Methane".GEOPHYSICAL RESEARCH LETTERS 50.16(2023):11.

入库方式: OAI收割

来源:广州地球化学研究所

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