中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Molecular and radiocarbon constraints on the fate of sedimentary organic carbon in a human-impacted river-dominated ocean margin

文献类型:期刊论文

作者Wang, Chenglong5; Zhang, Chuchu5; Zhang, Zhuoyue5; Liao, Qihang1,5; Zhang, Yang4,5; Wang, Ning2,3; Wang, Yaping5; Zou, Xinqing1,5
刊名MARINE GEOLOGY
出版日期2024-07-01
卷号473页码:12
关键词River -dominated Ocean margins Hydrodynamic sorting Human perturbations Mineral protection Molecular biomarkers Dual carbon isotope
ISSN号0025-3227
DOI10.1016/j.margeo.2024.107322
英文摘要Organic carbon (OC) burial in river-dominated ocean margins plays a pivotal role in the global carbon cycle, impacting atmospheric CO2 levels over the long term. Despite its significance, uncertainties persist regarding the influence of external environmental factors and intrinsic properties on sedimentary OC. In this study, we conducted a comprehensive analysis of surface sediments from the East China Sea, examining geochemical properties (including total OC content [TOC], Delta C-14, delta C-13, and C/N ratio), terrestrial biomarkers (n-alkanes), and mineral properties (such as specific surface area, Al/Si ratio, and mineral composition). Our aim was to shed light on the fate of sedimentary OC. The surface sediment's Delta C-14 values displayed significant spatial heterogeneity, delineating four distinct sub-regions. Strong positive correlations (all p < 0.01) were found between the triangle C-14 values and fine-grained sediments, specific surface area, and clay minerals, suggesting the potentially pivotal role of mineral protection in shaping the fate of sedimentary OC. The proportion of terrestrial OC gradually decreased towards the south, while marine OC proportion increased, corresponding to the enrichment of Delta C-14. The co-variation of Delta C-14 values, mineral properties, and OC source proportions suggests that terrestrial OC may undergo progressive replacement by marine OC during southward transport. Temporal variations in triangle C-14 values indicated that seabed erosion led to a significant increase in triangle C-14 values (p < 0.01) in the coastal mud belt, a phenomenon likely common in river-dominated ocean margins globally due to the new sediment cycle during the Anthropocene.
WOS研究方向Geology ; Oceanography
语种英语
WOS记录号WOS:001249370300001
源URL[http://ir.gig.ac.cn/handle/344008/78441]  
专题同位素地球化学国家重点实验室
通讯作者Zou, Xinqing
作者单位1.Nanjing Univ, Collaborat Innovat Ctr South China Sea Studies, Nanjing, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, CAS Ctr Excellence Deep Earth Sci, State Key Lab Isotope Geochem, Guangzhou 510640, Peoples R China
3.Southern Marine Sci & Engn Guangdong Lab Guangzhou, Guangzhou 511458, Peoples R China
4.Nanjing Univ, Sch Earth Sci & Engn, State Key Lab Mineral Deposits Res, Nanjing, Peoples R China
5.Nanjing Univ, Sch Geog & Oceanog Sci, Minist Educ, Key Lab Coast & Isl Dev, Nanjing, Peoples R China
推荐引用方式
GB/T 7714
Wang, Chenglong,Zhang, Chuchu,Zhang, Zhuoyue,et al. Molecular and radiocarbon constraints on the fate of sedimentary organic carbon in a human-impacted river-dominated ocean margin[J]. MARINE GEOLOGY,2024,473:12.
APA Wang, Chenglong.,Zhang, Chuchu.,Zhang, Zhuoyue.,Liao, Qihang.,Zhang, Yang.,...&Zou, Xinqing.(2024).Molecular and radiocarbon constraints on the fate of sedimentary organic carbon in a human-impacted river-dominated ocean margin.MARINE GEOLOGY,473,12.
MLA Wang, Chenglong,et al."Molecular and radiocarbon constraints on the fate of sedimentary organic carbon in a human-impacted river-dominated ocean margin".MARINE GEOLOGY 473(2024):12.

入库方式: OAI收割

来源:广州地球化学研究所

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