New insight into removal of tetracycline by a two-dimensional graphene-like carbon adsorbent prepared using one-step pyrolysis of spent bleaching earth: Adsorption behaviors, mechanisms and cost analysis
文献类型：期刊论文
| 作者 | Zhao, Ning1,5; Ma, Qiyi1,5; Zhang, Baifa3,4; Liu, Dong1,5 ; Wei, Yanfu2; Li, Mengyuan1,5; Yu, Ting1,5; Li, Haoyu1,5; Shen, Yuguo1,5; Yuan, Peng4
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| 刊名 | SEPARATION AND PURIFICATION TECHNOLOGY
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| 出版日期 | 2023-12-15 |
| 卷号 | 327页码:10 |
| 关键词 | Spent bleaching earth Electron energy loss spectroscopy Montmorillonite Two-dimensional graphene materials Tetracycline adsorption |
| ISSN号 | 1383-5866 |
| DOI | 10.1016/j.seppur.2023.124950 |
| 英文摘要 | Two-dimensional (2-D) graphene materials have high adsorption capacity for tetracycline because of great specific surface areas and abundant oxygen containing functional groups. Yet their application remains limited because of high costs and complex production processes. Here, a simple strategy for preparing 2-D graphene-like materials is proposed; spent bleaching earth (SBE), a by-product of bleaching edible oil, was initially used to prepare the 2-D material. Residual oils and minerals in SBE comprised the carbon sources and templates required for the 2-D material. The properties of SBE were utilized to synthesize mineral carbon material (SBE@C). This 2-D material (0.34-nm thickness) was investigated by checking the distribution of carbon in the SBE@C interlayer, using electron energy loss spectroscopy (EELS) in a scanning transmission electron microscope. The SBE@C's resulting 2-D graphene-like structure had an extraordinary uptake capacity for both tetracycline (96.48 mg/g) and sulfamethoxazole (94.24 mg/g). Further, the adsorbent featured excellent stability vis -`a-vis the competitive cationic coexistence, an extensive range of pH conditions, and multiple recycled uses (3 times), and its high-performance tetracycline adsorption from a real aquatic environment was also evidenced. Spectroscopic and microscopic studies showed that multiple adsorption mechanisms are involved, namely surface complexation, ion exchange, H-bond interaction, and pi-pi stacking. |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:001078452100001 |
| 源URL | [http://ir.gig.ac.cn/handle/344008/74902]  |
| 专题 | 中国科学院矿物学与成矿学重点实验室 |
| 通讯作者 | Yuan, Peng |
| 作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Macau Univ Sci & Technol, Macao Environm Res Inst, Natl Observat & Res Stn Coastal Ecol Environm Maca, Macau 999078, Peoples R China 3.Guangdong Univ Technol, Inst Environm Hlth & Pollut Control, Guangdong Key Lab Environm Catalysis & Hlth Risk C, Guangdong Hong Kong Macao Joint Lab Contaminants E, Guangzhou 510006, Peoples R China 4.Guangdong Univ Technol, Sch Environm Sci & Engn, Guangzhou 510006, Peoples R China 5.Chinese Acad Sci, Guangzhou Inst Geochem, CAS Key Lab Mineral & Metallogeny, Guangdong Prov Key Lab Mineral Phys & Mat, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Ning,Ma, Qiyi,Zhang, Baifa,et al. New insight into removal of tetracycline by a two-dimensional graphene-like carbon adsorbent prepared using one-step pyrolysis of spent bleaching earth: Adsorption behaviors, mechanisms and cost analysis[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2023,327:10. |
| APA | Zhao, Ning.,Ma, Qiyi.,Zhang, Baifa.,Liu, Dong.,Wei, Yanfu.,...&Yuan, Peng.(2023).New insight into removal of tetracycline by a two-dimensional graphene-like carbon adsorbent prepared using one-step pyrolysis of spent bleaching earth: Adsorption behaviors, mechanisms and cost analysis.SEPARATION AND PURIFICATION TECHNOLOGY,327,10. |
| MLA | Zhao, Ning,et al."New insight into removal of tetracycline by a two-dimensional graphene-like carbon adsorbent prepared using one-step pyrolysis of spent bleaching earth: Adsorption behaviors, mechanisms and cost analysis".SEPARATION AND PURIFICATION TECHNOLOGY 327(2023):10. |
入库方式： OAI收割
来源：广州地球化学研究所
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