中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Engineering a hard sol-gel adaptive coating with nonleaching antifoulant against marine biofouling in static conditions

文献类型:期刊论文

作者Sun, Yihan2; Shen, Yuanyuan2; Zhao, Haibin2; Wang, Peng2
刊名PROGRESS IN ORGANIC COATINGS
出版日期2024-06-01
卷号191页码:9
关键词Antifouling Fouling release Biofouling Low surface energy Coating
ISSN号0300-9440
DOI10.1016/j.porgcoat.2024.108402
通讯作者Wang, Peng(wangpeng@qdio.ac.cn)
英文摘要Covalently tethered, nonleaching antifoulant groups to surface or coating matrix are being explored as an ecofriendly option to develop a robust antifouling coating with enhanced static antifouling ability. And most of marine antifouling coatings usually have a relatively low coating hardness owing to intrinsically polymeric property. In this work, we exploited the self-assembly of random zwitterionic amphiphilic copolymers with an isothiazolinone-based antifoulant to develop a scalable hard (> 6H pencil hardness) coating against marine biofouling under static conditions. Upon exposure to aqueous media, strong fluorinate-zwitterion interactions drive microphase separation into bicontinuous networks of hydrophobic and zwitterionic nanodomains, leading to the enrichment of antifoulant moieties on the coating surface. The obtained hybrid coating could significantly restrain the growth of bacteria biofilms, the settlement of marine diatoms and mussel larvae owing to the presence of covalently tethered antifoulants. Oxidative stress levels in the body of bacteria and marine diatoms were significantly enhanced nearby the coating containing nonteaching antifoulants. On the other hand, the fouling release capability was not compromising on the developed hybrid coating with such high Young's modulus and large coating hardness, implying an obviously different antifouling mechanism. We attempt to report an ecofriendly and hard coating system to simultaneously prohibit fouling settlement and promote fouling removal in static conditions.
WOS关键词FOULING-RELEASE COATINGS ; ADHESION ; COPOLYMERS ; BIOCIDES ; IMPACT
资助项目National Natural Science Foundation of China[52205227] ; National Natural Science Foundation of China[U22A20112] ; Shandong Province Natural Science Foundation[ZR2020KE008] ; Nantong Scientific Plan Foundation[JC12022099]
WOS研究方向Chemistry ; Materials Science
语种英语
WOS记录号WOS:001219080000001
出版者ELSEVIER SCIENCE SA
源URL[http://ir.qdio.ac.cn/handle/337002/185673]  
专题海洋研究所_海洋腐蚀与防护研究发展中心
通讯作者Wang, Peng
作者单位1.Chinese Acad Sci, Ctr Ocean Mega Sci, Qingdao 266071, Peoples R China
2.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714
Sun, Yihan,Shen, Yuanyuan,Zhao, Haibin,et al. Engineering a hard sol-gel adaptive coating with nonleaching antifoulant against marine biofouling in static conditions[J]. PROGRESS IN ORGANIC COATINGS,2024,191:9.
APA Sun, Yihan,Shen, Yuanyuan,Zhao, Haibin,&Wang, Peng.(2024).Engineering a hard sol-gel adaptive coating with nonleaching antifoulant against marine biofouling in static conditions.PROGRESS IN ORGANIC COATINGS,191,9.
MLA Sun, Yihan,et al."Engineering a hard sol-gel adaptive coating with nonleaching antifoulant against marine biofouling in static conditions".PROGRESS IN ORGANIC COATINGS 191(2024):9.

入库方式: OAI收割

来源:海洋研究所

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