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  4. 中科院海岸带环境过程与生态修复重点实验室
Real-world emission characteristics of VOCs from typical cargo ships and their potential contributions to secondary organic aerosol and O3 under low-sulfur fuel policies

文献类型：期刊论文

作者Zhang, Fan2,3,4; Xiao, Binyu2; Liu, Zeyu5; Zhang, Yan1,6; Tian, Chongguo7; Li, Rui2,4; Wu, Can2,4; Lei, Yali8; Zhang, Si2,4; Wan, Xinyi2
刊名ATMOSPHERIC CHEMISTRY AND PHYSICS
出版日期2024-08-16
卷号24期号:16页码:8999-9017
ISSN号1680-7316
DOI10.5194/acp-24-8999-2024
通讯作者Zhang, Yan(yan_zhang@fudan.edu.cn) ; Wang, Gehui(ghwang@geo.ecnu.edu.cn)
英文摘要Mandatory use of low-sulfur fuel according to the global sulfur limit regulation has reduced the emissions of SO2 and particulate matter (PM) significantly on ships, and it also leads to a very large uncertainty in volatile organic compound (VOC) emissions. Therefore, an on-board test of VOCs from nine typical cargo ships with low-sulfur fuels in China was carried out in this study. Results showed that the emission factor of VOCs (EFVOCs) varied largely from 0.09 to 3.01 g kg(-1) of fuel, with domestic coastal cargo ships (CCSs) having the highest level, followed by inland cargo ships (ICSs) and ocean-going vessels (OGVs). The switch of fuels from heavy fuel oil (HFO) to diesel increased EFVOCs by 48 % on average, which enhanced both O-3 and secondary organic aerosol (SOA) formation potential, especially for OGVs. Besides, the use of low-sulfur fuels for OGVs also led to a significant increase in naphthalene emission. These indicated that the implementation of a global ultra-low-sulfur oil policy in the near future needs to be optimized. Moreover, aromatics were the most important common contributors to O-3 and SOA in ship exhausts, which need to be controlled as a matter of priority. It was also found that the benzene, toluene, and ethylbenzene ratio of 0.5: 0.3: 0.2 on average could be considered a diagnostic characteristic to distinguish ship emissions from other emission sources.
WOS关键词PEARL RIVER DELTA ; SHIPPING EMISSIONS ; CHEMICAL-COMPOSITION ; PARTICULATE MATTER ; GASEOUS EMISSIONS ; AIR-QUALITY ; DIESEL ; VEHICLES ; OZONE ; HYDROCARBON
WOS研究方向Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences
语种英语
WOS记录号WOS:001292394700001
资助机构National Natural Science Foundation of China ; State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex ; Ministry of Industry and Information Technology of China
源URL[http://ir.yic.ac.cn/handle/133337/35785]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_近岸生态与环境实验室
通讯作者Zhang, Yan; Wang, Gehui
作者单位1.Shanghai Inst Pollut Control & Ecol Secur, Shanghai 200092, Peoples R China
2.East China Normal Univ, Sch Geog Sci, Minist Educ, Key Lab Geog Informat Sci, Shanghai 200241, Peoples R China
3.Shanghai Acad Environm Sci, State Environm Protect Key Lab Format & Prevent U, Shanghai 200233, Peoples R China
4.Inst EcoChongming, 20 Cuiniao Rd, Shanghai 202162, Peoples R China
5.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess, Xian 710061, Peoples R China
6.Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Pre, Shanghai 200438, Peoples R China
7.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
8.Shanghai Environm Monitoring Ctr, State Ecol & Environm Sci Observat & Res Stn Yang, Shanghai 200030, Peoples R China
9.Hong Kong Polytech Univ, Dept Civil & Environm Engn, Kowloon, Hong Kong 100872, Peoples R China
10.Hong Kong Polytech Univ, State Key Lab Marine Pollut, Kowloon, Hong Kong 100872, Peoples R China
推荐引用方式
GB/T 7714		 Zhang, Fan,Xiao, Binyu,Liu, Zeyu,et al. Real-world emission characteristics of VOCs from typical cargo ships and their potential contributions to secondary organic aerosol and O3 under low-sulfur fuel policies[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2024,24(16):8999-9017.
APA Zhang, Fan.,Xiao, Binyu.,Liu, Zeyu.,Zhang, Yan.,Tian, Chongguo.,...&Wang, Gehui.(2024).Real-world emission characteristics of VOCs from typical cargo ships and their potential contributions to secondary organic aerosol and O3 under low-sulfur fuel policies.ATMOSPHERIC CHEMISTRY AND PHYSICS,24(16),8999-9017.
MLA Zhang, Fan,et al."Real-world emission characteristics of VOCs from typical cargo ships and their potential contributions to secondary organic aerosol and O3 under low-sulfur fuel policies".ATMOSPHERIC CHEMISTRY AND PHYSICS 24.16(2024):8999-9017.

入库方式： OAI收割

来源：烟台海岸带研究所

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