中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 烟台海岸带研究所
  3. 中国科学院烟台海岸带研究所
  4. 中科院海岸带环境过程与生态修复重点实验室
Ship Emissions as the Largest Contributor to Coastal Atmospheric Black Carbon at a Receptor Island in Southern China

文献类型：期刊论文

作者Geng, Xiaofei1,4,5; Li, Jun1,4,5; Zhong, Guangcai1,4,5; Zhao, Shizhen1,4,5; Tian, Chongguo3; Zhang, Yan-Lin2; Zhang, Gan1,4,5
刊名ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS
出版日期2024-06-13
页码7
关键词black carbon (BC) char-BC soot-BC ship emissions coastal aerosols sources
ISSN号2328-8930
DOI10.1021/acs.estlett.4c00362
通讯作者Zhang, Gan(zhanggan@gig.ac.cn)
英文摘要Atmospheric black carbon (BC) over coastal regions poses a threat in terms of both climate change and human health. However, the provenance of aerosol BC, particularly its subfractions (char-BC and soot-BC, which have different physicochemical properties), is poorly constrained. Here, we apportioned the sources of char-BC and soot-BC in year-round PM2.5 samples from a coastal receptor island off southern China. Char-BC dominated, accounting for 88.6 +/- 13.2% of the total BC. The two BC subfractions exhibited distinct seasonal variation patterns, which may be attributed to differences in their sources and hydrophilicity. Combustion of liquid fossil fuels, including bunker fuel, diesel, and gasoline, contributed more highly to soot-BC (71.4%) than to char-BC (53.9%). Conversely, combustion of solid fuels, including biomass and coal, contributed more highly to char-BC (44.6%) than to soot-BC (6.7%). Bunker fuel combustion, the dominant portion of ship emissions, was the largest contributor to total BC (46.0%), char-BC (45.2%), and soot-BC (56.4%). This indicates that marine ship emissions, rather than land-based sources including biomass and coal combustion, were the dominant source of atmospheric BC in coastal areas, highlighting the importance of controlling maritime ship emissions.
WOS关键词MOLECULAR MARKER ; ORGANIC AEROSOL ; BIOMASS ; SEA ; OUTFLOW ; TRACERS ; VESSELS ; EXHAUST ; METHANE ; METALS
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
WOS记录号WOS:001247368400001
资助机构National Natural Science Foundation of China ; National Natural Science Foundation of China ; Alliance of International Science Organizations ; Youth Innovation Promotion Association of CAS ; China Postdoctoral Science Foundation ; NASA's Earth Observing System Data and Information System (EOSDIS)
源URL[http://ir.yic.ac.cn/handle/133337/35920]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_近岸生态与环境实验室
通讯作者Zhang, Gan
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China
2.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Nanjing 214111, Peoples R China
3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
4.Guangdong Prov Key Lab Environm Protect & Resource, Guangzhou 510640, Peoples R China
5.Guangdong Hong Kong Macao Joint Lab Environm Pollu, Guangzhou 510640, Peoples R China
推荐引用方式
GB/T 7714		 Geng, Xiaofei,Li, Jun,Zhong, Guangcai,et al. Ship Emissions as the Largest Contributor to Coastal Atmospheric Black Carbon at a Receptor Island in Southern China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS,2024:7.
APA Geng, Xiaofei.,Li, Jun.,Zhong, Guangcai.,Zhao, Shizhen.,Tian, Chongguo.,...&Zhang, Gan.(2024).Ship Emissions as the Largest Contributor to Coastal Atmospheric Black Carbon at a Receptor Island in Southern China.ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS,7.
MLA Geng, Xiaofei,et al."Ship Emissions as the Largest Contributor to Coastal Atmospheric Black Carbon at a Receptor Island in Southern China".ENVIRONMENTAL SCIENCE & TECHNOLOGY LETTERS (2024):7.

入库方式： OAI收割

来源：烟台海岸带研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。