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Diffusive gradients in thin films (DGT) probe for effectively sampling of per- and polyfluoroalkyl substances in waters and sediments

文献类型：期刊论文

作者Yang, Yuanyuan1,3; Liu, Sisi1,3; Wang, Runmei2; Li, Cailin1,3; Tang, Jianhui2; Chen, Tao1,3; Ying, Guang-Guo1,3; Chen, Chang-Er1,3
刊名JOURNAL OF ENVIRONMENTAL SCIENCES
出版日期2022-11-01
卷号121页码:90-97
关键词Diffusive gradients in thin films (DGT) Passive sampling Per- and polyfluoroalkyl substances (PFAS) Sediment Aquatic environments
ISSN号1001-0742
DOI10.1016/j.jes.2021.09.003
通讯作者Wang, Runmei(rmwang@yic.ac.cn) ; Chen, Chang-Er(changer.chen@m.scnu.edu.cn)
英文摘要The passive sampling technique, diffusive gradients in thin films (DGT) has attracted increasing interests as an in-situ sampler for organic contaminants including per- and polyfluoroalkyl substances (PFAS). However, its effectiveness has been questioned because of the small effective sampling area (3.1 cm(2)). In this study, we developed a DGT probe for rapid sampling of eight PFAS in waters and applied it to a water-sediment system. It has a much larger sampling area (27 cm(2)) and as a result lower method quantification limits (0.15 - 0.21 ng/L for one-day deployment and 0.02 - 0.03 ng/L for one-week deployment) and much higher (by > 10 factors) sampling rate (100 mL/day) compared to the standard DGT (piston configuration). The sampler could linearly accumulate PFAS from wastewater, was sensitive enough even for a 24 hr deployment with performance comparable to grab sampling (500 mL). The DGT probe provided homogeneous sampling performance along the large exposure area. The use of the probe to investigate distributions of dissolved PFAS around the sediment-water interface was demonstrated. This work, for the first time, demonstrated that the DGT probe is a promising monitoring tool for trace levels of PFAS and a research tool for studying their distribution, migration, and fate in aquatic environments including the sediment-water interface. (C) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
WOS关键词IN-SITU MEASUREMENT ; ORGANIC CONTAMINANTS ; PERFLUOROALKYL ACIDS ; TRACE-METALS ; MOBILIZATION
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000800545000010
资助机构Key Deployment Project of Centre for Ocean Mega-Research of Science, Chinese Academy of Sciences ; Guangzhou Municipal Science and Technology Project ; National Natural Science Foundation of China ; Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety
源URL[http://ir.yic.ac.cn/handle/133337/37517]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_近岸生态与环境实验室
通讯作者Wang, Runmei; Chen, Chang-Er
作者单位1.South China Normal Univ, MOE Key Lab Theoret Chem Environm, Guangzhou 510006, Peoples R China
2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
3.South China Normal Univ, Environm Res Inst, Sch Environm, Guangdong Prov Key Lab Chem Pollut & Environm Saf, Guangzhou 510006, Peoples R China
推荐引用方式
GB/T 7714		 Yang, Yuanyuan,Liu, Sisi,Wang, Runmei,et al. Diffusive gradients in thin films (DGT) probe for effectively sampling of per- and polyfluoroalkyl substances in waters and sediments[J]. JOURNAL OF ENVIRONMENTAL SCIENCES,2022,121:90-97.
APA Yang, Yuanyuan.,Liu, Sisi.,Wang, Runmei.,Li, Cailin.,Tang, Jianhui.,...&Chen, Chang-Er.(2022).Diffusive gradients in thin films (DGT) probe for effectively sampling of per- and polyfluoroalkyl substances in waters and sediments.JOURNAL OF ENVIRONMENTAL SCIENCES,121,90-97.
MLA Yang, Yuanyuan,et al."Diffusive gradients in thin films (DGT) probe for effectively sampling of per- and polyfluoroalkyl substances in waters and sediments".JOURNAL OF ENVIRONMENTAL SCIENCES 121(2022):90-97.

入库方式： OAI收割

来源：烟台海岸带研究所

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