Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent
文献类型:期刊论文
作者 | Li, Yanhua4; Wu, Long1,2,3,4; Xu, Qing1,2,4; Li, Zhanyong1,4 |
刊名 | JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT
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出版日期 | 2022-08-16 |
页码 | 12 |
关键词 | CaO-based biochar Crab shell Sewage sludge Steam gasification H-2-rich syngas |
ISSN号 | 1438-4957 |
DOI | 10.1007/s10163-022-01480-z |
通讯作者 | Wu, Long(wulong@tust.edu.cn) |
英文摘要 | A CaO-based biochar (CSC) prepared from waste crab shell was used as a low-cost CO2 sorbent to enhance sludge steam gasification for H-2-rich gas production. The effects of gasification temperature and CSC addition on sludge gasification performance were investigated. Results showed that the sludge steam gasification can be evidently enhanced with CSC addition and produced H-2-rich gas with CO2 removal. The appropriate gasification temperature for CSC sorption-enhanced gasification should be below 800 celcius. With CSC addition at 700 celcius, H-2 content increased to 63.2% (36.4% of pure sludge case) while CO2 content reduced to 3.5% (34.5% of pure sludge case). Meanwhile, the H-2-rich syngas with high H-2/CO ratio (up to 10.2) was achieved. At higher gasification temperature of 800 celcius and 900 celcius, the CO2 absorbed in the CSC will be released via the decomposition reaction of CaCO3 and adding CSC showed slight effect on sludge gasification. Although the Ca content in CSC was less than 36%, CSC showed almost the same positive effects on H-2 production and CO2 reduction compared to pure CaO in sludge gasification process. These findings indicated that CSC has the potential to replace CaO for sorption-enhanced gasification for sewage sludge disposal. |
WOS关键词 | SEWAGE-SLUDGE ; STEAM GASIFICATION ; CALCIUM-OXIDE ; BIOMASS |
资助项目 | CAS Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion ; Key Area Research and Development Program of Guangdong Province[2020B0202010004] |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
WOS记录号 | WOS:000841060800002 |
出版者 | SPRINGER |
资助机构 | CAS Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion ; Key Area Research and Development Program of Guangdong Province |
源URL | [http://ir.giec.ac.cn/handle/344007/37129] ![]() |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Wu, Long |
作者单位 | 1.Int Joint Res Ctr Low Carbon Green Proc Equipment, Tianjin 300222, Peoples R China 2.Guangdong Intelligent Filling Technol Ltd Co, Guangzhou 510640, Peoples R China 3.Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Tianjin Univ Sci & Technol, Coll Mech Engn, Tianjin Key Lab Integrated Design & On Line Monit, Tianjin 300222, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Yanhua,Wu, Long,Xu, Qing,et al. Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent[J]. JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT,2022:12. |
APA | Li, Yanhua,Wu, Long,Xu, Qing,&Li, Zhanyong.(2022).Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent.JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT,12. |
MLA | Li, Yanhua,et al."Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent".JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT (2022):12. |
入库方式: OAI收割
来源:广州能源研究所
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