中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent

文献类型:期刊论文

作者Li, Yanhua4; Wu, Long1,2,3,4; Xu, Qing1,2,4; Li, Zhanyong1,4
刊名JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT
出版日期2022-08-16
页码12
关键词CaO-based biochar Crab shell Sewage sludge Steam gasification H-2-rich syngas
ISSN号1438-4957
DOI10.1007/s10163-022-01480-z
通讯作者Wu, Long(wulong@tust.edu.cn)
英文摘要A CaO-based biochar (CSC) prepared from waste crab shell was used as a low-cost CO2 sorbent to enhance sludge steam gasification for H-2-rich gas production. The effects of gasification temperature and CSC addition on sludge gasification performance were investigated. Results showed that the sludge steam gasification can be evidently enhanced with CSC addition and produced H-2-rich gas with CO2 removal. The appropriate gasification temperature for CSC sorption-enhanced gasification should be below 800 celcius. With CSC addition at 700 celcius, H-2 content increased to 63.2% (36.4% of pure sludge case) while CO2 content reduced to 3.5% (34.5% of pure sludge case). Meanwhile, the H-2-rich syngas with high H-2/CO ratio (up to 10.2) was achieved. At higher gasification temperature of 800 celcius and 900 celcius, the CO2 absorbed in the CSC will be released via the decomposition reaction of CaCO3 and adding CSC showed slight effect on sludge gasification. Although the Ca content in CSC was less than 36%, CSC showed almost the same positive effects on H-2 production and CO2 reduction compared to pure CaO in sludge gasification process. These findings indicated that CSC has the potential to replace CaO for sorption-enhanced gasification for sewage sludge disposal.
WOS关键词SEWAGE-SLUDGE ; STEAM GASIFICATION ; CALCIUM-OXIDE ; BIOMASS
资助项目CAS Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion ; Key Area Research and Development Program of Guangdong Province[2020B0202010004]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000841060800002
出版者SPRINGER
资助机构CAS Key Laboratory of Renewable Energy, Guangzhou Institute of Energy Conversion ; Key Area Research and Development Program of Guangdong Province
源URL[http://ir.giec.ac.cn/handle/344007/37129]  
专题中国科学院广州能源研究所
通讯作者Wu, Long
作者单位1.Int Joint Res Ctr Low Carbon Green Proc Equipment, Tianjin 300222, Peoples R China
2.Guangdong Intelligent Filling Technol Ltd Co, Guangzhou 510640, Peoples R China
3.Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
4.Tianjin Univ Sci & Technol, Coll Mech Engn, Tianjin Key Lab Integrated Design & On Line Monit, Tianjin 300222, Peoples R China
推荐引用方式
GB/T 7714
Li, Yanhua,Wu, Long,Xu, Qing,et al. Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent[J]. JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT,2022:12.
APA Li, Yanhua,Wu, Long,Xu, Qing,&Li, Zhanyong.(2022).Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent.JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT,12.
MLA Li, Yanhua,et al."Hydrogen-rich gas production from sorption-enhanced sludge gasification using CaO-based biochar derived from crab shell as a CO2 sorbent".JOURNAL OF MATERIAL CYCLES AND WASTE MANAGEMENT (2022):12.

入库方式: OAI收割

来源:广州能源研究所

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