Municipal sludge derived solid acids for levoglucosenone production via cellulose fast pyrolysis
文献类型：期刊论文
| 作者 | Yuan, Haoran2,3,4,5,6 ; Li, Chengyu2,3,5,6; Shan, Rui2,3,4,5,6; Zhang, Jun2,3,4,6; Zhu, Lingjun1; Chen, Yong2,3,4,5,6
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| 刊名 | JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS
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| 出版日期 | 2022-10-01 |
| 卷号 | 167页码:8 |
| 关键词 | Municipal sludge Solid acids Pyrolysis Levoglucosenone |
| ISSN号 | 0165-2370 |
| DOI | 10.1016/j.jaap.2022.105663 |
| 通讯作者 | Zhang, Jun(zhangjun@ms.giec.ac.cn) |
| 英文摘要 | In the present study, a series of municipal sludge derived solid acids, synthesized through hydrothermal pre-carbonization coupled with secondary pyrolysis method, were developed for levoglucosenone (LGO) production via cellulose fast pyrolysis. Specific physico-chemical characterizations such as XRD, FTIR, N-2 adsorption-desorption, NH3-TPD, etc., were undertaken to reveal the structural properties of as-prepared solid acids. Phosphoric acid and sulfuric acid decorated municipal sludge derived carbon-based materials containing abundant Bronsted acid sites remarkably facilitated the selective formation of LGO. Particularly, high LGO yield (similar to 20 wt%) were achieved using both phosphoric and sulfonic acid functionalized municipal sludge derived porous carbon. The as-prepared municipal sludge derived solid acids could be reused for multiple cycles in LGO preparation without significant decline in pyrolysis performance. This research will provide good reference for the resource utilization of lignocellulosic biomass and municipal sludge, particularly in the aspect of valuable chemicals manufacture. |
| WOS关键词 | LIGNOCELLULOSIC BIOMASS ; BIO-OIL ; MECHANISM ; PHOSPHORYLATION ; TEMPERATURE ; INSIGHT |
| 资助项目 | National Key R & D Program of China[2018YFC1901200] ; National Natural Science Foundation of China[51976222] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou)[GML2019ZD0101] ; Guangdong Basic and Applied Basic Research Foundation[2021B1515020068] ; State Key Laboratory of Clean Energy Utilization[ZJU-CEU2020023] |
| WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000868332100004 |
| 出版者 | ELSEVIER |
| 资助机构 | National Key R & D Program of China ; National Natural Science Foundation of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) ; Guangdong Basic and Applied Basic Research Foundation ; State Key Laboratory of Clean Energy Utilization |
| 源URL | [http://ir.giec.ac.cn/handle/344007/37565]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Zhang, Jun |
| 作者单位 | 1.Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Peoples R China 2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 4.Southern Marine Sci & Engn Guangdong Lab Guangzhou, Zhuhai 511458, Peoples R China 5.Univ Sci & Technol China, Sch Energy Sci & Engn, Guangzhou 510640, Peoples R China 6.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yuan, Haoran,Li, Chengyu,Shan, Rui,et al. Municipal sludge derived solid acids for levoglucosenone production via cellulose fast pyrolysis[J]. JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,2022,167:8. |
| APA | Yuan, Haoran,Li, Chengyu,Shan, Rui,Zhang, Jun,Zhu, Lingjun,&Chen, Yong.(2022).Municipal sludge derived solid acids for levoglucosenone production via cellulose fast pyrolysis.JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS,167,8. |
| MLA | Yuan, Haoran,et al."Municipal sludge derived solid acids for levoglucosenone production via cellulose fast pyrolysis".JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS 167(2022):8. |
入库方式： OAI收割
来源：广州能源研究所
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