Mapping Dissolved Gases Distribution in Lake Water Using Shipborne Membrane Inlet Mass Spectrometry
文献类型：期刊论文
| 作者 | Wang, Han; Liu, Chang-jie; Song, Hai-yun; Liu, You-jiang ; Chen, Chi-lai
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| 刊名 | CHINESE JOURNAL OF ANALYTICAL CHEMISTRY
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| 出版日期 | 2024-07-01 |
| 卷号 | 52 |
| 关键词 | Membrane inlet mass spectrometer Dissolved gases Online detection Algae |
| ISSN号 | 0253-3820 |
| DOI | 10.19756/j.issn.0253-3820.241010 |
| 通讯作者 | Chen, Chi-lai(chlchen@iim.ac.cn) |
| 英文摘要 | As global average carbon dioxide concentrations steadily rise, the frequency, intensity, and duration of cyanobacterial blooms in aquatic ecosystems are increasing annually. This phenomenon presents a significant threat to the overall health of global ecosystems and has garnered worldwide attention. In this study, an online detection of small-molecule dissolved gas concentrations in lake using a home-made-made membrane inlet mass spectrometer was conducted. Comparative water samples analyses demonstrated that the developed mass spectrometer instrument effectively discriminated between different water samples based on its dissolved gas detection capabilities. Online survey revealed that the concentrations of dissolved O-2 and dissolved CO2 were 0.24 mmol/L and 1.31 mu mol/L, respectively, in areas without cyanobacterial coverage. In areas with cyanobacterial coverage, their concentrations were 0.21 mmol/L and 0.92 mu mol/L, respectively. In areas where cyanobacteria were densely collected, the dissolved CO2 content rose rapidly, while the dissolved O-2 content decreased rapidly. This result revealed that large-scale-scale cyanobacterial blooms exacerbated CO2 emissions, and during such blooms, lakes acted as sources of CO2, emitting substantial amounts into the atmosphere, thereby contributing to adverse impacts on global climate change. Furthermore, extensive cyanobacterial blooms led to a rapid decrease in dissolved O-2 levels, resulting in O-2 depletion and the mortality of fish and benthic invertebrates. The research highlighted the significance of the ratio of content of O-2 and CO2 as a crucial indicator for cyanobacterial monitoring, with a smaller ratio indicating higher cyanobacterial content. Moreover, changes in turbidity and variations in the ratio of O-2 and CO2 exhibited strong consistency. Large-scale-scale algal blooms increased water turbidity, which posed a threat to the survival of aquatic organisms. This study provided a technological means for online detection of dissolved gases in water, offering essential references for water quality assessment, ecological evaluation, and particularly, for early prevention, mid-term-term management, and post-treatment effectiveness assessment of cyanobacterial blooms. |
| WOS关键词 | IN-SITU ANALYSIS ; CARBON ; METHANE ; ONLINE ; FIELD |
| 资助项目 | National Key R&D Program of China[2021YFC2800301] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA22020503] ; Instrument Developing Project of Chinese Academy of Sciences[YJKYYQ20210008] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:001301307300001 |
| 出版者 | SCIENCE PRESS |
| 资助机构 | National Key R&D Program of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Instrument Developing Project of Chinese Academy of Sciences |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/134902]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Chen, Chi-lai |
| 作者单位 | Chinese Acad Sci, Hefei Inst Phys Sci, Hefei 230031, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Han,Liu, Chang-jie,Song, Hai-yun,et al. Mapping Dissolved Gases Distribution in Lake Water Using Shipborne Membrane Inlet Mass Spectrometry[J]. CHINESE JOURNAL OF ANALYTICAL CHEMISTRY,2024,52. |
| APA | Wang, Han,Liu, Chang-jie,Song, Hai-yun,Liu, You-jiang,&Chen, Chi-lai.(2024).Mapping Dissolved Gases Distribution in Lake Water Using Shipborne Membrane Inlet Mass Spectrometry.CHINESE JOURNAL OF ANALYTICAL CHEMISTRY,52. |
| MLA | Wang, Han,et al."Mapping Dissolved Gases Distribution in Lake Water Using Shipborne Membrane Inlet Mass Spectrometry".CHINESE JOURNAL OF ANALYTICAL CHEMISTRY 52(2024). |
入库方式： OAI收割
来源：合肥物质科学研究院
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