中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Mid-infrared optical frequency comb-based Fourier transform spectrometer for broadband molecular spectroscopy

文献类型:期刊论文

作者Cheng, Feihu1; Zhao, Weixiong1; Fang, Bo1; Yang, Nana1; Li, Shuangshuang1; Zhang, Weijun1; Deng, Lunhua2,3; Chen, Weidong4
刊名CHINESE JOURNAL OF CHEMICAL PHYSICS
出版日期2024-08-01
卷号37
关键词Mid-infrared optical frequency comb Multi-pass cell Fourier transform infrared spectrometer
ISSN号1674-0068
DOI10.1063/1674-0068/cjcp2401007
通讯作者Zhao, Weixiong(wxzhao@aiofm.ac.cn)
英文摘要Optical freciuency comb-based Fourier transform spectroscopy has the features of broad spectral bandwidth, high sensitivity, and multiplexed trace gas detection, which has valuable application potential in the fields of precision spectroscopy and trace gas detection. Here, we report the development of a mid-infrared Fourier transform spectrometer based on an optical frequency comb combined with a Herriott-type multipass cell. Using this instrument, the broadband absorption spectra of several important molecules, including methane, acetylene, water molecules and nitrous oxide, are measured by near real-time data acquisition in the 2800-3500 cm(-1) spectral region. The achieved minimum detectable absorption of the instrument is 4.4xl0(-8) cm(-1)Hz(-1//2) per spectral element. Broadband spectra of H2O are fitted using the Voigt profile multispectral fitting technique and the consistency of the concentration inversion is 1%. Our system also enables precise spectroscopic measurements, and it allows the determination of the spectral line positions and upper state constants of N2O in the (0002)-(1000) band, with results in good agreement with those reported by Toth [Appl. Opt. 30, 5289 (1991)].
WOS关键词MU-M ; RESOLUTION ; PROGRAM ; N2O
资助项目National Natural Science Foundation of China[42022051] ; National Natural Science Foundation of China[U21A2028] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[Y202089] ; HFIPS Director's Fund[YZJJ202101] ; HFIPS Director's Fund[BJPY2023A02]
WOS研究方向Physics
语种英语
WOS记录号WOS:001286620100014
出版者CHINESE PHYSICAL SOC
资助机构National Natural Science Foundation of China ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; HFIPS Director's Fund
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/135016]  
专题中国科学院合肥物质科学研究院
通讯作者Zhao, Weixiong
作者单位1.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Lab Atmospher Phys Chem, HFIPS, Hefei 230031, Peoples R China
2.East China Normal Univ, State Key Lab Precis Spect, Shanghai 200062, Peoples R China
3.East China Normal Univ, Dept Phys, Shanghai 200062, Peoples R China
4.Univ Littoral Cote dOpale, Lab Phys Chim Atmosphere, F-59140 Dunkerque, France
推荐引用方式
GB/T 7714
Cheng, Feihu,Zhao, Weixiong,Fang, Bo,et al. Mid-infrared optical frequency comb-based Fourier transform spectrometer for broadband molecular spectroscopy[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2024,37.
APA Cheng, Feihu.,Zhao, Weixiong.,Fang, Bo.,Yang, Nana.,Li, Shuangshuang.,...&Chen, Weidong.(2024).Mid-infrared optical frequency comb-based Fourier transform spectrometer for broadband molecular spectroscopy.CHINESE JOURNAL OF CHEMICAL PHYSICS,37.
MLA Cheng, Feihu,et al."Mid-infrared optical frequency comb-based Fourier transform spectrometer for broadband molecular spectroscopy".CHINESE JOURNAL OF CHEMICAL PHYSICS 37(2024).

入库方式: OAI收割

来源:合肥物质科学研究院

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