Multi-deformable interpenetrating network thermosensitive hydrogel fluorescent device for real-time and visual detection of nitrite
文献类型：期刊论文
| 作者 | Li, Lingfei1; Lin, Dan1,2; Xu, Shihao1,2; Yang, Liang1,2; Jiang, Changlong1,2
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| 刊名 | JOURNAL OF HAZARDOUS MATERIALS
 |
| 出版日期 | 2024-10-05 |
| 卷号 | 478 |
| 关键词 | Ratiometric sensing Visual detection Hydrogel materials Interpenetrating network Food safety Nitrite |
| ISSN号 | 0304-3894 |
| DOI | 10.1016/j.jhazmat.2024.135471 |
| 通讯作者 | Yang, Liang(yangliang@iim.ac.cn) ; Jiang, Changlong(cljiang@iim.ac.cn) |
| 英文摘要 | Functionalized thermosensitive hydrogel materials exhibit excellent properties for the fabrication of sensing devices that enable real-time visual detection of food safety duo to their good plasticity and powerful loading capacity. Here, a ratiometric fluorescent device based on an interpenetrating network (IPN) thermosensitive hydrogel was designed to embed functionalized Au nanoclusters (Au NCs) and Blue Carbon dots (BCDs) composites in a multi-network structure to build a sensitive hazardous material nitrite (NO2- ) chemsensor. The hydrogel was utilized poloxamer 407 (P407), lignin and cellulose to form stable IPN structure, which resulted in complementation and synergy, thereby strengthening its porous network structure. The combination of fluorescent nanoprobes with the porous network structure has the potential to enhance stable fluorescence signals and improve sensing sensitivity. Moreover, the thermosensitive liquid-solid transition characteristics of the hydrogel facilitate its preparation into diverse sensing devices following curing at room temperature. The hydrogel device, when combined with a smartphone system, converted image information into data information, thereby enabling the accurate quantification of NO2 - with a detection limit of 9.38 nM in 2 s. The designed multifunctional hydrogel device is capable of real-time differentiation of NO2 - dosage with the naked eye, offering a high-contrast, rapid-response sensing methodology for visual assessment of food freshness. This research contributes to the expansion of hydrogel materials applications and the detection of hazardous materials in food safety. |
| WOS关键词 | CARBON NANODOTS ; NANOPARTICLES ; NANOCLUSTERS ; EMISSION ; NITRATE ; MEAT |
| 资助项目 | National Key Research and Development Program[2021YFD2000202] ; National Natural Science Foundation of China[22274158] ; Natural Science Foundation of Anhui Provincial[2208085MB30] ; Anhui Provincial Key Research |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:001296942500001 |
| 出版者 | ELSEVIER |
| 资助机构 | National Key Research and Development Program ; National Natural Science Foundation of China ; Natural Science Foundation of Anhui Provincial ; Anhui Provincial Key Research |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/135890]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Yang, Liang; Jiang, Changlong |
| 作者单位 | 1.Chinese Acad Sci, Inst Solid State Phys, Hefei Inst Phys Sci, Hefei 230031, Anhui, Peoples R China 2.Chinese Acad Sci, State Key Lab Transducer Technol, Hefei 230031, Anhui, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Lingfei,Lin, Dan,Xu, Shihao,et al. Multi-deformable interpenetrating network thermosensitive hydrogel fluorescent device for real-time and visual detection of nitrite[J]. JOURNAL OF HAZARDOUS MATERIALS,2024,478. |
| APA | Li, Lingfei,Lin, Dan,Xu, Shihao,Yang, Liang,&Jiang, Changlong.(2024).Multi-deformable interpenetrating network thermosensitive hydrogel fluorescent device for real-time and visual detection of nitrite.JOURNAL OF HAZARDOUS MATERIALS,478. |
| MLA | Li, Lingfei,et al."Multi-deformable interpenetrating network thermosensitive hydrogel fluorescent device for real-time and visual detection of nitrite".JOURNAL OF HAZARDOUS MATERIALS 478(2024). |
入库方式： OAI收割
来源：合肥物质科学研究院
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